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中国黑龙江省露天生物质燃烧更高分辨率多年排放清单的编制。

Development of a finer-resolution multi-year emission inventory for open biomass burning in Heilongjiang Province, China.

作者信息

Li Bin, Xu Zehua, Liu Baiyin, Zhang Zhimiao, Qiu Wenting, Wang Wei

机构信息

Institute of Environmental Information, Chinese Research Academy of Environmental Sciences, Beijing, China.

出版信息

Sci Rep. 2024 Dec 2;14(1):29969. doi: 10.1038/s41598-024-81092-9.

Abstract

Open biomass burning (OBB) is a significant source of air pollutants, profoundly impacting regional air quality and global climate change. However, due to the lack of high-resolution burned area products, limited biomass data resolution, and inappropriate emission factors (EFs), current OBB emission inventories have significant uncertainties. In this study, we integrated the FireCCI51 burned area product (250 m), high-resolution gridded biomass data, localized EFs, and various statistical survey data to compile a finer-resolution (250 m) and long-term (2001-2020) inventory of 11 pollutants for Heilongjiang Province (an important agricultural and forestry region in China). The results indicated that the annual average OBB emissions in Heilongjiang Province were 12.26, 63.70, 931.60, 17,203.35, 16.09, 171.25, 39.83, 71.22, 184.33, 129.16, and 6.35 Gg for BC, CH, CO, CO, NH, NMVOC, NOx, OC, PM, PM, and SO, respectively. Taking PM as an example, emissions from cropland, forest, and grassland burning accounted for 73%, 26%, and 1% respectively. Geographically, emissions were primarily concentrated in the western, southwestern, and northeastern regions of Heilongjiang. The peak PM2.5 emissions exhibited notable seasonal variation, with maxima occurring in April and October. This is primarily due to the extensive burning of straw during the spring and autumn ploughing seasons. The results of this study provide a detailed multi-year inventory crucial for atmospheric transport models and can support the development of effective pollution control strategies and greenhouse gas mitigation measures.

摘要

露天生物质燃烧(OBB)是空气污染物的重要来源,对区域空气质量和全球气候变化产生深远影响。然而,由于缺乏高分辨率的燃烧面积产品、生物质数据分辨率有限以及排放因子(EFs)不合适,当前的OBB排放清单存在很大的不确定性。在本研究中,我们整合了FireCCI51燃烧面积产品(250米)、高分辨率网格化生物质数据、本地化排放因子以及各种统计调查数据,编制了黑龙江省(中国重要的农林地区)分辨率更高(250米)且为期较长(2001 - 2020年)的11种污染物排放清单。结果表明,黑龙江省OBB的年平均排放量分别为:黑碳(BC)12.26Gg、甲烷(CH)63.70Gg、一氧化碳(CO)931.60Gg、二氧化碳(CO₂)17203.35Gg、氨(NH₃)16.09Gg、非甲烷挥发性有机物(NMVOC)171.25Gg、氮氧化物(NOₓ)39.83Gg、有机碳(OC)71.22Gg、细颗粒物(PM₂.₅)184.33Gg、可吸入颗粒物(PM₁₀)129.16Gg、二氧化硫(SO₂)6.35Gg。以PM₂.₅为例,农田、森林和草地燃烧排放分别占73%、26%和1%。从地理位置上看,排放主要集中在黑龙江省的西部、西南部和东北部地区。PM₂.₅排放峰值呈现出显著的季节变化,最大值出现在4月和10月。这主要是由于春秋季耕地季节大量焚烧秸秆所致。本研究结果提供了一份详细的多年排放清单,对大气传输模型至关重要,并可为制定有效的污染控制策略和温室气体减排措施提供支持。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b30b/11612381/2c2dd7f345b3/41598_2024_81092_Fig1_HTML.jpg

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