Liu Min, Lei Yunze, Yu Lan, Fang Xiang, Ma Ying, Liu Lixin, Zheng Juanjuan, Gao Peng
School of Physics, Xidian University, Xi'an 710071, China.
Guangzhou Institute of Technology, Xidian University, Guangzhou 510555, China.
Nanophotonics. 2022 Jun 27;11(15):3395-3420. doi: 10.1515/nanoph-2022-0241. eCollection 2022 Aug.
Super-resolution optical microscopy, which gives access to finer details of objects, is highly desired for fields of nanomaterial, nanobiology, nanophotonics, etc. Many efforts, including tip optimization and illumination optimization etc., have been made in both near-field and far-field super-resolution microscopy to achieve a spatial resolution beyond the diffraction limit. The development of vector light fields opens up a new avenue for super-resolution optical microscopy via special illumination modes. Cylindrical vector beam (CVB) has been verified to enable resolution improvement in tip-scanning imaging, nonlinear imaging, stimulated emission depletion (STED) microscopy, subtraction imaging, superoscillation imaging, etc. This paper reviews recent advances in CVB-based super-resolution imaging. We start with an introduction of the fundamentals and properties of CVB. Next, strategies for CVB based super-resolution imaging are discussed, which are mainly implemented by tight focusing, depletion effect, plasmonic nanofocusing, and polarization matching. Then, the roadmap of super-resolution imaging with CVB illumination in the past two decades is summarized. The typical CVB-based imaging techniques in fields of both near-field and far-field microscopy are introduced, including tip-scanning imaging, nonlinear imaging, STED, subtraction imaging, and superoscillation imaging. Finally, challenges and future directions of CVB-illuminated super-resolution imaging techniques are discussed.
超分辨率光学显微镜能够获取物体更精细的细节,在纳米材料、纳米生物学、纳米光子学等领域有着极高的需求。在近场和远场超分辨率显微镜中,人们已经做出了许多努力,包括针尖优化和照明优化等,以实现超越衍射极限的空间分辨率。矢量光场的发展通过特殊的照明模式为超分辨率光学显微镜开辟了一条新途径。圆柱矢量光束(CVB)已被证实能够在针尖扫描成像、非线性成像、受激辐射损耗(STED)显微镜、相减成像、超振荡成像等方面提高分辨率。本文综述了基于CVB的超分辨率成像的最新进展。我们首先介绍CVB的基本原理和特性。接下来,讨论基于CVB的超分辨率成像策略,这些策略主要通过紧聚焦、损耗效应、等离子体纳米聚焦和偏振匹配来实现。然后,总结了过去二十年中使用CVB照明的超分辨率成像的发展历程。介绍了近场和远场显微镜领域中典型的基于CVB的成像技术,包括针尖扫描成像、非线性成像、STED、相减成像和超振荡成像。最后,讨论了CVB照明超分辨率成像技术面临的挑战和未来发展方向。