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用于快速定时应用的等离子体紫外线滤光片。

Plasmonic ultraviolet filter for fast-timing applications.

作者信息

Ota Ryosuke, Uenoyama Soh

机构信息

Central Research Laboratory, Hamamatsu Photonics K.K., 5000 Hirakuchi, Hamakita-ku, Hamamatsu City 434-8601, Japan.

出版信息

Nanophotonics. 2023 Jan 23;12(4):743-752. doi: 10.1515/nanoph-2022-0704. eCollection 2023 Feb.

Abstract

Barium fluoride, an inorganic scintillation material used for the detection of X-ray and/or gamma-ray radiation, has been receiving increasing attention in the field of radiation measurements in fast-timing applications. To make full use of its timing properties, its slow emission around the ultraviolet region, more specifically, the 300 nm region needs to be suppressed. Although doping ions, such as lanthanum, yttrium, and cadmium, can suppress the slow component, such techniques can lose information of interacted radiations. Consequently, a suppression technique that does not suffer from information loss while maintaining precise timing measurements would be desirable. In this study, we proposed aluminum nano-disk-based plasmonic filters to suppress slow emissions while maintaining fast emissions around 195 and 220 nm and a usability of the slow component. Finite-difference time-domain simulations and experimental results exhibited good agreement, with over 90% of slow components being adequately suppressed without sacrificing fast components, proving that aluminum nanodisks can be used for ultraviolet filters. Moreover, based on the designed filter performance, we conducted coincidence time resolution simulations for positron-electron annihilation gamma rays from an analytical perspective. The simulations indicated the designed filters could maintain high timing performance. Consequently, the proposed plasmonic ultraviolet filter was suitable for maximizing the potential of barium fluoride scintillators.

摘要

氟化钡是一种用于检测X射线和/或γ射线辐射的无机闪烁材料,在快速计时应用的辐射测量领域中受到越来越多的关注。为了充分利用其计时特性,需要抑制其在紫外区域(更具体地说是300nm区域)的缓慢发射。虽然诸如镧、钇和镉等掺杂离子可以抑制慢成分,但这些技术可能会丢失相互作用辐射的信息。因此,需要一种在保持精确计时测量的同时不会出现信息丢失的抑制技术。在本研究中,我们提出了基于铝纳米盘的等离子体滤波器,以抑制缓慢发射,同时保持195和220nm附近的快速发射以及慢成分的可用性。时域有限差分模拟和实验结果显示出良好的一致性,超过90%的慢成分得到充分抑制,而不牺牲快成分,证明铝纳米盘可用于紫外滤波器。此外,基于设计的滤波器性能,我们从分析角度对正电子-电子湮灭γ射线进行了符合时间分辨率模拟。模拟表明,设计的滤波器可以保持高计时性能。因此,所提出的等离子体紫外滤波器适用于最大化氟化钡闪烁体的潜力。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3f6f/11636206/a925b0cfac83/j_nanoph-2022-0704_fig_001.jpg

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