Research Laboratory of Electronics, Massachusetts Institute of Technology, Cambridge, MA 02139, USA.
Department of Physics, Massachusetts Institute of Technology, Cambridge, MA 02139, USA.
Science. 2022 Feb 25;375(6583):eabm9293. doi: 10.1126/science.abm9293.
Bombardment of materials by high-energy particles often leads to light emission in a process known as scintillation. Scintillation has widespread applications in medical imaging, x-ray nondestructive inspection, electron microscopy, and high-energy particle detectors. Most research focuses on finding materials with brighter, faster, and more controlled scintillation. We developed a unified theory of nanophotonic scintillators that accounts for the key aspects of scintillation: energy loss by high-energy particles, and light emission by non-equilibrium electrons in nanostructured optical systems. We then devised an approach based on integrating nanophotonic structures into scintillators to enhance their emission, obtaining nearly an order-of-magnitude enhancement in both electron-induced and x-ray-induced scintillation. Our framework should enable the development of a new class of brighter, faster, and higher-resolution scintillators with tailored and optimized performance.
高能粒子轰击材料通常会导致发光,这一过程被称为闪烁。闪烁在医学成像、X 射线无损检测、电子显微镜和高能粒子探测器等领域有广泛的应用。大多数研究都集中在寻找发光更亮、更快、更可控的材料上。我们提出了一个纳米光子闪烁体的统一理论,该理论考虑了闪烁的关键方面:高能粒子的能量损失,以及纳米结构光学系统中非平衡电子的发光。然后,我们设计了一种将纳米光子结构集成到闪烁体中的方法来增强其发光,从而在电子和 X 射线诱导的闪烁中获得近一个数量级的增强。我们的框架应该能够开发出一类新的闪烁体,它们具有更高的亮度、更快的速度和更高的分辨率,并且具有可定制和优化的性能。