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高性能FeO/rGO/TiO纳米催化剂处理亚甲基蓝染料和大肠杆菌废水

Treatment of Wastewater from Methylene Blue Dye and E. Coli Bacteria by High-Performance FeO/rGO/TiO Nanocatalyst.

作者信息

Sanjari Mahjube, Molaei Mehdi, Seifi Akram, Iranmanesh Parvaneh, Farahmandzadeh Farzad

机构信息

Department of Physics, Faculty of Science, Vali-e-Asr University of Rafsanjan, Rafsanjan, Iran.

Department of Water Science & Engineering, Faculty of Agriculture, Vali-e-Asr University of Rafsanjan, Rafsanjan, Iran.

出版信息

J Fluoresc. 2024 Dec 16. doi: 10.1007/s10895-024-04067-z.

Abstract

Photocatalysis-based technology has insight into decreasing the disadvantages of traditional approaches and has been identified as an appropriate way to eliminate dyes and bacteria from wastewater. In this work, FeO/rGO/TiO photocatalyst material was synthesized by a simple and fast hydrothermal method. The photocatalyst process results showed that FeO/rGO/TiO nanocomposite degraded methylene blue dye completely in 4 min. Also, FeO/rGO/TiO nanocomposite was very efficient (4.92 log reduction value) for E. Coli bacteria inactivation in 60 min photocatalyst process. The superparamagnetic behavior of FeO/rGO/TiO nanocomposite was investigated by VSM analysis and magnetization saturation was obtained at about 38.46 emu/g which gives simple and fast separation from media to FeO/rGO/TiO nanocatalyst. The structural and morphology properties of FeO/rGO/TiO nanocomposite were studied by XRD, Raman, FT-IR, EDS, FESEM, and TEM analysis. The obtained results confirmed that FeO/rGO/TiO nanocomposite is an efficient nanocatalyst for the treatment of MB dye and E. Coli. Bacteria from water, simultaneously.

摘要

基于光催化的技术有助于减少传统方法的缺点,并且已被视为从废水中去除染料和细菌的一种合适方法。在这项工作中,通过简单快速的水热法合成了FeO/rGO/TiO光催化剂材料。光催化过程结果表明,FeO/rGO/TiO纳米复合材料在4分钟内完全降解了亚甲基蓝染料。此外,在60分钟的光催化过程中,FeO/rGO/TiO纳米复合材料对大肠杆菌的灭活非常有效(对数减少值为4.92)。通过VSM分析研究了FeO/rGO/TiO纳米复合材料的超顺磁行为,获得的磁化饱和度约为38.46 emu/g,这使得从介质中简单快速分离出FeO/rGO/TiO纳米催化剂成为可能。通过XRD、拉曼、FT-IR、EDS、FESEM和TEM分析研究了FeO/rGO/TiO纳米复合材料的结构和形貌特性。所得结果证实,FeO/rGO/TiO纳米复合材料是一种同时处理水中MB染料和大肠杆菌的高效纳米催化剂。

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