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微滴从表面重新悬浮

Microdroplet Resuspension Off Surfaces.

作者信息

Wu Yue, Islam Khayrul, Liu Yaling, Jagota Anand

机构信息

Department of Chemical and Biomolecular Engineering, Lehigh University, 19 Memorial Drive West, Bethlehem, Pennsylvania 18015, United States.

Department of Bioengineering, Lehigh University, 19 Memorial Drive West, Bethlehem, Pennsylvania 18015, United States.

出版信息

Langmuir. 2024 Dec 31;40(52):27206-27215. doi: 10.1021/acs.langmuir.4c02833. Epub 2024 Dec 16.

Abstract

Understanding the resuspension of droplets from surfaces into air is important for elucidating a range of processes such as disease transmission of airborne pathogens and determining environmental contamination and the effectiveness of cleaning procedures. The resuspension condition is defined as the escape velocity of a droplet from a surface. This study investigated the dynamics of microliter-sized droplet resuspension off surfaces utilizing a novel free-fall device. We studied surfaces with three different wettabilities, three droplet volumes, and substrate velocities ranging from 0 to 3.5 m/s for deionized water and viscous droplets representing a prototype saliva substitute. Experimental results provide quantitative results for the increased propensity for drop resuspension for more hydrophobic surfaces, larger droplet volume, and higher velocity. By using high-speed imaging, we segment the resuspension process into four stages: initial equilibrium, deformation, elongation, and breakage. Experimental results are generalized as a machine-learning-derived decision surface, which predicts resuspension by defining a 2D decision boundary in our 3D parameter space. We present a simple physical model, corroborated by computational fluid dynamics simulations, for the dynamics of resuspension that explains the process and is in good agreement with the experiments.

摘要

了解液滴从表面重新悬浮到空气中的过程,对于阐明一系列过程至关重要,例如空气传播病原体的疾病传播、确定环境污染以及清洁程序的有效性。重新悬浮条件被定义为液滴从表面逸出的速度。本研究利用一种新型自由落体装置研究了微升大小液滴从表面重新悬浮的动力学。我们研究了具有三种不同润湿性、三种液滴体积以及去离子水和代表原型唾液替代品的粘性液滴在0至3.5米/秒范围内的基底速度的表面。实验结果为疏水性更强的表面、更大的液滴体积和更高的速度下液滴重新悬浮倾向增加提供了定量结果。通过高速成像,我们将重新悬浮过程分为四个阶段:初始平衡、变形、伸长和破裂。实验结果被归纳为一个机器学习衍生的决策面,该决策面通过在我们的三维参数空间中定义二维决策边界来预测重新悬浮。我们提出了一个简单的物理模型,该模型得到计算流体动力学模拟的证实,用于重新悬浮动力学,解释了该过程并与实验结果高度吻合。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f3d5/11697350/0a2b092cd33b/la4c02833_0001.jpg

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