Yue Shuai, Zhao Zhiyong, Zhang Tao, Li Fei, Wang Pengfei, Zhan Sihui
MOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Remediation and Pollution Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, P. R. China.
Environ Sci Technol. 2024 Dec 31;58(52):22865-22879. doi: 10.1021/acs.est.4c06688. Epub 2024 Dec 17.
The extensive accumulation of plastic waste has given rise to severe environmental pollution issues. Contemporary conventional recycling methods, such as incineration and landfilling, contribute significantly to pollutant emissions and carbon footprints, against the principles of sustainable development. Leveraging renewable solar energy to transform plastics into high-value chemicals and green fuels offers a more promising and sustainable approach to managing plastic waste resources. This comprehensive review centers on the recent advancements in plastic photoreforming, categorizing them based on the types of end products. Particular emphasis is placed on the evolving research landscape surrounding the conversion of plastics into high-value chemicals through photoreforming, as well as the economic considerations for large-scale photoreforming production. The analysis conducted here reveals key pathways and emerging trends that are poised to shape the trajectory of enhanced photoconversion, ultimately influencing the realization of a carbon-neutral future.
塑料垃圾的大量积累引发了严重的环境污染问题。当代传统回收方法,如焚烧和填埋,对污染物排放和碳足迹有很大影响,违背了可持续发展原则。利用可再生太阳能将塑料转化为高价值化学品和绿色燃料,为管理塑料废物资源提供了一种更有前景和可持续的方法。本综述围绕塑料光催化重整的最新进展展开,根据最终产品类型对其进行分类。特别强调了通过光催化重整将塑料转化为高价值化学品的不断发展的研究领域,以及大规模光催化重整生产的经济考量。此处进行的分析揭示了关键途径和新兴趋势,这些趋势将塑造增强光催化转化的轨迹,最终影响碳中和未来的实现。