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揭示中国长江三角洲南部地区大气微塑料的季节性传输及暴露风险。

Unveiling the seasonal transport and exposure risks of atmospheric microplastics in the southern area of the Yangtze River Delta, China.

作者信息

Nafea Taiseer Hussain, Shun Chan Faith Ka, Xu Yuyao, Xiao Hang, He Jun

机构信息

Department of Chemical and Environmental Engineering, University of Nottingham Ningbo China, Ningbo, China; Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, China.

School of Geographical Sciences, University of Nottingham Ningbo China, Ningbo, China.

出版信息

Environ Pollut. 2025 Feb 15;367:125567. doi: 10.1016/j.envpol.2024.125567. Epub 2024 Dec 20.

Abstract

This study investigates the prevalence and impacts of suspended atmospheric microplastics (SAMPs) in the coastal metropolitan city of Ningbo in the Yangtze River Delta Region, China. The sampling was conducted at both urban centre and urban-rural fringe areas, near the coast but distant from large urban populations. SAMP abundance ranged from 0.017 to 0.430 items m³, with an average of 0.145 ± 0.09 items m⁻³. The urban centre exhibited approximately 70% more SAMPs than the urban-rural fringe, highlighting the influence of population density and human activity on microplastic pollution. Fibres dominated SAMP composition at both sites, while urban samples featured a greater variety of microplastic forms, such as fragments, beads, and films. Rayon and Polyethylene terephthalate were the predominant polymers, which were found to be directly related to local industrial activities. SAMPs ranged in size from 20 μm to 4984.4 μm, with over 60% smaller than 1000 μm. Seasonal variation followed a winter > autumn > spring > summer pattern. Correlation and principal component analyses identified atmospheric temperature, pressure, wind speed, and rainfall as key factors influencing SAMP abundance. Notably, backward trajectory analysis showed that oceanic air masses carried significantly fewer SAMPs compared to terrestrial air, diluting concentrations in coastal regions. Annually, an estimated 4.67 × 10³ microplastics are suspended over Ningbo. This is the first comprehensive study of SAMP pollution in this region, revealing interactions between local sources, environmental variations, air mass dynamics, and exposure. The findings underscore the need for targeted strategies to mitigate atmospheric microplastic pollution in coastal urban environments.

摘要

本研究调查了中国长江三角洲地区沿海大都市宁波大气中悬浮微塑料(SAMPs)的污染程度及其影响。采样点位于城市中心和城乡边缘地区,靠近海岸但远离大城市人口密集区。SAMPs的丰度范围为0.017至0.430个/立方米,平均为0.145±0.09个/立方米。城市中心的SAMPs含量比城乡边缘地区高出约70%,突出了人口密度和人类活动对微塑料污染的影响。两个采样点的SAMP成分均以纤维为主,而城市样本中的微塑料形态更为多样,如碎片、珠子和薄膜。人造丝和聚对苯二甲酸乙二酯是主要聚合物,发现它们与当地工业活动直接相关。SAMPs的尺寸范围为20微米至4984.4微米,超过60%小于1000微米。季节变化呈现冬季>秋季>春季>夏季的模式。相关性和主成分分析确定气温、气压、风速和降雨是影响SAMP丰度的关键因素。值得注意的是,后向轨迹分析表明,与陆地气团相比,海洋气团携带的SAMPs明显较少,从而稀释了沿海地区的浓度。据估计,宁波每年有4.67×10³个微塑料悬浮在空中。这是该地区首次对SAMP污染进行的全面研究,揭示了本地源、环境变化、气团动态和暴露之间的相互作用。研究结果强调了制定针对性策略以减轻沿海城市环境中大气微塑料污染的必要性。

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