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中国东部沿海大气中的微塑料:不同功能区反映不同来源和传输途径。

Microplastics in the atmospheric of the eastern coast of China: different function areas reflecting various sources and transport.

机构信息

College of Ecology Environment and Urban Construction, Fujian University of Technology, Fuzhou, 350108, China.

State Key Laboratory of Marine Environmental Science, Xiamen University, Xiamen, 361102, China.

出版信息

Environ Geochem Health. 2024 Oct 1;46(11):461. doi: 10.1007/s10653-024-02217-7.

Abstract

Suspended atmospheric microplastics (SAMPs) display varying occurrence characteristics on different underlying surfaces in urban areas. This study investigated the occurrence characteristics, source apportionment, and transportation patterns of SAMPs in two typical underlying surfaces: the downtown area (Site T) and the industrial area (Site C) of a coastal city in China. In the spring of 2023, a total of 32 types comprising 1325 SAMPs were detected. The average MP abundances were found to be 3.74 ± 2.86 n/m in Site T and 2.67 ± 1.68 n/m in Site C. In Site T, SAMPs attributed to living source constituted 78.05%, while industry was the main source in Site C with a proportion reaching 42.89%, consistent with the functional zoning of the underlying surface. Furthermore, HYSPLIT analysis revealed that there was no significant difference between these two sites in long-distance horizontal transport affected by external airflow regardless of altitude; conversely, PCA indicated a notable correlation between vertical velocity and both abundance and species diversity. According to the hourly average wind speeds, the maximum transmission distance was computed as 350 km for updraft and the minimum transmission distances was as low as 32 m for downdraft. Subsequently, the coincidence between the source proportion of SAMPs on random day and meteorological parameters confirmed the synergistic impact on SAMPs transport influenced by functional zoning, geographic environment, and vertical velocity.

摘要

悬浮大气中的微塑料(SAMPs)在城市不同的下垫面具有不同的出现特征。本研究调查了中国沿海城市两个典型下垫面(市区 T 点和工业区 C 点)中 SAMPs 的出现特征、来源分配和传输模式。2023 年春季,共检测到 32 种,包含 1325 个 SAMPs。T 点的平均 MPs 丰度为 3.74±2.86 n/m,C 点的为 2.67±1.68 n/m。在 T 点,来源于生活源的 SAMPs 占 78.05%,而 C 点的主要来源是工业,占比达到 42.89%,与下垫面的功能分区一致。此外,HYSPLIT 分析表明,无论海拔如何,受外部气流影响的长距离水平传输在这两个站点之间没有显著差异;相反,PCA 表明垂直速度与丰度和物种多样性之间存在显著相关性。根据每小时平均风速,上升气流的最大传输距离计算为 350 公里,下降气流的最小传输距离低至 32 米。随后,随机日 SAMPs 来源比例与气象参数的一致性证实了功能分区、地理环境和垂直速度对 SAMPs 传输的协同影响。

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