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二维半导体异质结构中层间激子超流性的成像

Imaging interlayer exciton superfluidity in a 2D semiconductor heterostructure.

作者信息

Cutshall Jacob, Mahdikhany Fateme, Roche Anna, Shanks Daniel N, Koehler Michael R, Mandrus David G, Taniguchi Takashi, Watanabe Kenji, Zhu Qizhong, LeRoy Brian J, Schaibley John R

机构信息

Department of Physics, University of Arizona, Tucson, AZ 85721, USA.

McCormick School of Engineering, Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208, USA.

出版信息

Sci Adv. 2025 Jan 3;11(1):eadr1772. doi: 10.1126/sciadv.adr1772.

DOI:10.1126/sciadv.adr1772
PMID:39752490
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11698081/
Abstract

Excitons, which are Coulomb bound electron-hole pairs, are composite bosons and thus at low temperature can form a superfluid state with a single well-defined amplitude and phase. We directly image this macroscopic exciton superfluid state in an hBN-separated MoSe-WSe heterostructure. At high density, we identify quasi-long-range order over the entire active area of our sample, through spatially resolved coherence measurements. By varying the exciton density and sample temperature, we map out the phase diagram of the superfluid. We observe the superfluid phase persisting to a temperature of 15 K, which is in excellent agreement with theoretical predictions. This works paves the way to realizing on chip superfluid structures capable of studying fundamental physical behaviors and quantum devices that use superfluidity.

摘要

激子是库仑束缚的电子 - 空穴对,属于复合玻色子,因此在低温下可形成具有单一明确振幅和相位的超流态。我们直接成像了hBN分离的MoSe - WSe异质结构中的这种宏观激子超流态。在高密度下,通过空间分辨相干测量,我们在样品的整个有源区域识别出准长程有序。通过改变激子密度和样品温度,我们绘制出了超流体的相图。我们观察到超流相持续到15 K的温度,这与理论预测非常吻合。这项工作为实现能够研究基本物理行为的芯片上超流体结构以及利用超流性的量子器件铺平了道路。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/40d2/11698081/4d50be80ff88/sciadv.adr1772-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/40d2/11698081/54619e91ddf1/sciadv.adr1772-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/40d2/11698081/46c8138a4320/sciadv.adr1772-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/40d2/11698081/d8318fd3ada0/sciadv.adr1772-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/40d2/11698081/4d50be80ff88/sciadv.adr1772-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/40d2/11698081/54619e91ddf1/sciadv.adr1772-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/40d2/11698081/46c8138a4320/sciadv.adr1772-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/40d2/11698081/d8318fd3ada0/sciadv.adr1772-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/40d2/11698081/4d50be80ff88/sciadv.adr1772-f4.jpg

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本文引用的文献

1
Long-distance decay-less spin transport in indirect excitons in a van der Waals heterostructure.范德华异质结构中间接激子的长距离无衰减自旋输运。
Nat Commun. 2024 Nov 1;15(1):9454. doi: 10.1038/s41467-024-53445-5.
2
Direct Visualization of Dark Interlayer Exciton Transport in Moiré Superlattices.莫尔超晶格中暗层间激子输运的直接可视化
Nano Lett. 2024 Jan 10;24(1):339-346. doi: 10.1021/acs.nanolett.3c04105. Epub 2023 Dec 26.
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Thermodynamic behavior of correlated electron-hole fluids in van der Waals heterostructures.范德华异质结构中关联电子-空穴流体的热力学行为
Nat Commun. 2023 Dec 13;14(1):8264. doi: 10.1038/s41467-023-43799-7.
4
Extended Spatial Coherence of Interlayer Excitons in MoSe_{2}/WSe_{2} Heterobilayers.二硒化钼/二硒化钨异质双层中层间激子的扩展空间相干性
Phys Rev Lett. 2023 Jul 21;131(3):036902. doi: 10.1103/PhysRevLett.131.036902.
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Electrical control of hybrid exciton transport in a van der Waals heterostructure.范德华异质结构中混合激子输运的电学控制
Nat Photonics. 2023;17(7):615-621. doi: 10.1038/s41566-023-01198-w. Epub 2023 Apr 20.
6
Localized interlayer excitons in MoSe-WSe heterostructures without a moiré potential.无莫尔势的MoSe-WSe异质结构中的局域层间激子
Nat Commun. 2022 Sep 12;13(1):5354. doi: 10.1038/s41467-022-33082-6.
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Interlayer Exciton Diode and Transistor.层间激子二极管与晶体管。
Nano Lett. 2022 Aug 24;22(16):6599-6605. doi: 10.1021/acs.nanolett.2c01905. Epub 2022 Aug 15.
8
Direct visualization of magnetic domains and moiré magnetism in twisted 2D magnets.扭曲二维磁体中磁畴和莫尔磁学的直接可视化
Science. 2021 Nov 26;374(6571):1140-1144. doi: 10.1126/science.abj7478. Epub 2021 Nov 25.
9
Excitons and emergent quantum phenomena in stacked 2D semiconductors.堆叠二维半导体中的激子和新兴量子现象。
Nature. 2021 Nov;599(7885):383-392. doi: 10.1038/s41586-021-03979-1. Epub 2021 Nov 17.
10
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Nature. 2021 Oct;598(7882):585-589. doi: 10.1038/s41586-021-03947-9. Epub 2021 Oct 27.