Mahdikhanysarvejahany Fateme, Shanks Daniel N, Klein Matthew, Wang Qian, Koehler Michael R, Mandrus David G, Taniguchi Takashi, Watanabe Kenji, Monti Oliver L A, LeRoy Brian J, Schaibley John R
Department of Physics, University of Arizona, Tucson, AZ, 85721, USA.
Guangdong Provincial Key Laboratory of Quantum Metrology and Sensing & School of Physics and Astronomy, Sun Yat-Sen University (Zhuhai Campus), Zhuhai, 519082, China.
Nat Commun. 2022 Sep 12;13(1):5354. doi: 10.1038/s41467-022-33082-6.
Interlayer excitons (IXs) in MoSe-WSe heterobilayers have generated interest as highly tunable light emitters in transition metal dichalcogenide (TMD) heterostructures. Previous reports of spectrally narrow (<1 meV) photoluminescence (PL) emission lines at low temperature have been attributed to IXs localized by the moiré potential between the TMD layers. We show that spectrally narrow IX PL lines are present even when the moiré potential is suppressed by inserting a bilayer hexagonal boron nitride (hBN) spacer between the TMD layers. We compare the doping, electric field, magnetic field, and temperature dependence of IXs in a directly contacted MoSe-WSe region to those in a region separated by bilayer hBN. The doping, electric field, and temperature dependence of the narrow IX lines are similar for both regions, but their excitonic g-factors have opposite signs, indicating that the origin of narrow IX PL is not the moiré potential.
作为过渡金属二硫属化物(TMD)异质结构中高度可调谐的发光体,MoSe-WSe异质双层中的层间激子(IXs)引起了人们的关注。先前关于低温下光谱窄(<1 meV)光致发光(PL)发射线的报道归因于TMD层之间的莫尔势局域化的IXs。我们表明,即使通过在TMD层之间插入双层六方氮化硼(hBN)间隔层来抑制莫尔势,光谱窄的IX PL线仍然存在。我们比较了直接接触的MoSe-WSe区域和由双层hBN隔开的区域中IXs的掺杂、电场、磁场和温度依赖性。两个区域中窄IX线的掺杂、电场和温度依赖性相似,但它们的激子g因子具有相反的符号,这表明窄IX PL的起源不是莫尔势。