Matsumura Shin, Shida Ayano, Tsuchii Moeno, Wada Mika, Charneau Jimmy, Tsuji Motonori, Hasumi Keiji, Suzuki Eriko
Department of Applied Biological Science, Tokyo University of Agriculture and Technology, Fuchu 183-8509, Japan.
Department of Research and Development, TMS Co., Fuchu 183-0055, Japan.
Int J Mol Sci. 2024 Dec 17;25(24):13496. doi: 10.3390/ijms252413496.
Soluble epoxide hydrolase (sEH) is a bifunctional enzyme with epoxide hydrolase activity in the C-terminal domain (C-EH) and lipid phosphate phosphatase activity in the N-terminal domain (N-phos). The C-EH hydrolyzes bioactive epoxy fatty acids such as epoxyeicosatrienoic acid (EET). The N-phos hydrolyzes lipid phosphomonesters, including the signaling molecules of lysophosphatidic acid (LPA). Here, we report that the C-EH and N-phos are reciprocally regulated by their respective substrates. Full-length sEH (sEH-FL) showed positive cooperativity toward the substrate for each domain. Similar cooperativity was found when truncated enzymes having only C- and N-terminal domains, sEH-C and sEH-N, respectively, were used, suggesting an intra-domain nature of the cooperativity. In addition, the N-phos substrate LPA inhibited C-EH activity in sEH-FL and sEH-C equally. Similarly, the C-EH substrate EET inhibited N-phos activity. Structural and kinetic data suggest the presence of allosteric sites in each domain of the sEH enzyme, which share the binding of LPA and EET. Thus, each of the two sEH activities is regulated by a substrate of its own and by that of the other domain. This mechanism may explain why sEH has evolved to have two different enzyme activities, which possibly allows sEH to balance the metabolism of bioactive lipids.
可溶性环氧化物水解酶(sEH)是一种双功能酶,其C末端结构域(C-EH)具有环氧化物水解酶活性,N末端结构域(N-phos)具有脂质磷酸酶活性。C-EH可水解生物活性环氧脂肪酸,如环氧二十碳三烯酸(EET)。N-phos可水解脂质磷酸单酯,包括溶血磷脂酸(LPA)的信号分子。在此,我们报告C-EH和N-phos受各自底物的相互调节。全长sEH(sEH-FL)对每个结构域的底物表现出正协同性。当分别使用仅具有C末端和N末端结构域的截短酶sEH-C和sEH-N时,也发现了类似的协同性,这表明协同性具有结构域内性质。此外,N-phos底物LPA同样抑制sEH-FL和sEH-C中的C-EH活性。同样,C-EH底物EET抑制N-phos活性。结构和动力学数据表明,sEH酶的每个结构域中都存在变构位点,这些位点共享LPA和EET的结合。因此,sEH的两种活性各自都受到其自身底物以及另一个结构域底物的调节。这种机制可能解释了为什么sEH进化出具有两种不同的酶活性,这可能使sEH能够平衡生物活性脂质的代谢。