Xiao Xue, Fu Yu, Zhang Daojing, Gao Shuhong
State Key Laboratory of Bioreactor Engineering, East China University of Science and Technology, Shanghai, 200237, China.
Bioprocess Biosyst Eng. 2025 Mar;48(3):493-507. doi: 10.1007/s00449-024-03124-y. Epub 2025 Jan 7.
Ascomycin (FK520) is a 23-membered macrolide antibiotic primarily produced by the Streptomyces hygroscopicus var. ascomyceticus. Structurally similar to tacrolimus and rapamycin, it serves as an effective immunosuppressant widely used in the treatment of rejection reactions after organ transplantation and certain autoimmune diseases. Currently, FK520 is mainly produced through microbial fermentation, but its yield remains low. Since the gene fkbR2 is a regulatory gene within the FK520 biosynthesis gene cluster that has not been studied, this paper focuses on the overexpression of the gene fkbR2 in Streptomyces hygroscopicus var. ascomyceticus ATCC 14891 (WT). By constructing a strain with overexpressed fkbR2 gene, we initially obtained a high-yield strain R2-17 through shake flask fermentation, with a 28% increase in yield compared to WT. In the process of further improving the stability of the high-yield strain, this paper defines two indices: high-yield index and stability index. After two consecutive rounds of natural breeding, strain R2-17 achieved a high-yield index of 100% and a stability index of 80%. Finally, the high-yield strain R2-17-3-10 was successfully screened, and the yield was increased by 34% compared with the strain WT, reaching 686.47 mg/L. A comparative analysis between the high-yield strain R2-17-3-10 and the original strain WT revealed differences in fermentation process parameters such as FK520 synthesis rate, pH, bacterial growth, glycerol consumption rate, ammonia nitrogen level, and ammonium ion concentration. In addition, the transcription levels of genes involved in the synthesis of precursors 4,5-dihydroxycyclohex-1-enecarboxylic acid (fkbO), ethylmalonyl-CoA (fkbE, fkbU, fkbS), and pipecolic acid (fkbL), as well as pathway-specific regulatory genes (fkbN, fkbR1), were significantly increased at different time points in the high-yield strain R2-17-3-10. EMSAs analysis showed that the FkbR2 protein could not bind to the promoter region of above genes. This suggests that the gene fkbR2 may enhance the supply of FK520 synthetic precursors by indirectly regulating the transcription levels of these genes, thereby promoting an increase in FK520 production. These results demonstrate that modifying genes within the biosynthetic gene clusters of natural products can be successfully applied to increase the yields of industrially and clinically important compounds. However, it is found that fkbR2 gene is a regulatory gene that has not been fully studied, and it is worth further studying its regulatory mechanism.
子囊霉素(FK520)是一种23元大环内酯类抗生素,主要由吸水链霉菌子囊菌变种产生。它在结构上与他克莫司和雷帕霉素相似,是一种有效的免疫抑制剂,广泛用于治疗器官移植后的排斥反应和某些自身免疫性疾病。目前,FK520主要通过微生物发酵生产,但其产量仍然较低。由于fkbR2基因是FK520生物合成基因簇中的一个尚未研究的调控基因,本文重点研究了fkbR2基因在吸水链霉菌子囊菌变种ATCC 14891(WT)中的过表达。通过构建fkbR2基因过表达菌株,我们通过摇瓶发酵初步获得了高产菌株R2-17,其产量比WT提高了28%。在进一步提高高产菌株稳定性的过程中,本文定义了两个指标:高产指标和稳定性指标。经过两轮连续的自然选育,菌株R2-17的高产指标达到100%,稳定性指标达到80%。最终成功筛选出高产菌株R2-17-3-10,其产量比WT菌株提高了34%,达到686.47mg/L。高产菌株R2-17-3-10与原始菌株WT的比较分析揭示了发酵过程参数的差异,如FK520合成速率、pH值、细菌生长、甘油消耗速率、氨氮水平和铵离子浓度。此外,在高产菌株R2-17-3-10的不同时间点,参与前体4,5-二羟基环己-1-烯羧酸(fkbO)、乙基丙二酰辅酶A(fkbE、fkbU、fkbS)和哌啶酸(fkbL)合成的基因以及途径特异性调控基因(fkbN、fkbR1)的转录水平显著提高。电泳迁移率变动分析表明,FkbR2蛋白不能与上述基因的启动子区域结合。这表明fkbR基因可能通过间接调节这些基因的转录水平来增强FK520合成前体的供应,从而促进FK520产量的增加。这些结果表明,修饰天然产物生物合成基因簇中的基因可以成功应用于提高工业和临床重要化合物的产量。然而,发现fkbR2基因是一个尚未充分研究的调控基因,其调控机制值得进一步研究。