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采用公民科学方法评估偏远高海拔冰川中的纳米塑料污染。

Using a citizen science approach to assess nanoplastics pollution in remote high-altitude glaciers.

作者信息

Jurkschat Leonie, Gill Alasdair J, Milner Robin, Holzinger Rupert, Evangeliou Nikolaos, Eckhardt Sabine, Materić Dušan

机构信息

Faculty of Chemistry and Mineralogy, Leipzig University, 04103, Leipzig, Germany.

Department of Environmental Analytical Chemistry, Helmholtz Centre for Environmental Research (UFZ), 04318, Leipzig, Germany.

出版信息

Sci Rep. 2025 Jan 13;15(1):1864. doi: 10.1038/s41598-024-84210-9.

DOI:10.1038/s41598-024-84210-9
PMID:39805969
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11729883/
Abstract

Nanoplastics are suspected to pollute every environment on Earth, including very remote areas reached via atmospheric transport. We approached the challenge of measuring environmental nanoplastics by combining high-sensitivity TD-PTR-MS (thermal desorption-proton transfer reaction-mass spectrometry) with trained mountaineers sampling high-altitude glaciers ("citizen science"). Particles < 1 μm were analysed for common polymers (polyethylene, polyethylene terephthalate, polypropylene, polyvinyl chloride, polystyrene and tire wear particles), revealing nanoplastic concentrations ranging 2-80 ng mL at five of 14 sites. The dominant polymer types found in this study were tire wear, polystyrene and polyethylene particles (41%, 28% and 12%, respectively). Lagrangian dispersion modelling was used to reconstruct possible sources of micro- and nanoplastic emissions for those observations, which appear to lie largely to the west of the Alps. France, Spain and Switzerland have the highest contributions to the modelled emissions. The citizen science approach was found to be feasible providing strict quality control measures are in place, and is an effective way to be able to collect data from remote and inaccessible regions across the world.

摘要

纳米塑料被怀疑污染地球上的每一个环境,包括通过大气传输到达的非常偏远的地区。我们通过将高灵敏度的热解吸-质子转移反应-质谱(TD-PTR-MS)与训练有素的登山者对高海拔冰川进行采样(“公民科学”)相结合,来应对测量环境中纳米塑料的挑战。对小于1微米的颗粒进行了常见聚合物(聚乙烯、聚对苯二甲酸乙二酯、聚丙烯、聚氯乙烯、聚苯乙烯和轮胎磨损颗粒)分析,在14个地点中的5个地点发现纳米塑料浓度范围为2 - 80纳克/毫升。本研究中发现的主要聚合物类型是轮胎磨损颗粒、聚苯乙烯颗粒和聚乙烯颗粒(分别占41%、28%和12%)。利用拉格朗日扩散模型重建了这些观测结果中微塑料和纳米塑料排放的可能来源,这些来源似乎主要位于阿尔卑斯山以西。法国、西班牙和瑞士对模拟排放的贡献最大。结果发现,只要有严格的质量控制措施,公民科学方法是可行的,并且是一种能够从世界各地偏远和难以到达的地区收集数据的有效方式。

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本文引用的文献

1
Fine micro- and nanoplastics concentrations in particulate matter samples from the high alpine site Sonnblick, Austria.奥地利高海拔索内布利克站点颗粒物样本中的微塑料和纳米塑料精细浓度。
Chemosphere. 2024 Mar;352:141410. doi: 10.1016/j.chemosphere.2024.141410. Epub 2024 Feb 10.
2
Shape Matters: Long-Range Transport of Microplastic Fibers in the Atmosphere.形状很重要:大气中微塑料纤维的长距离传输。
Environ Sci Technol. 2024 Jan 9;58(1):671-682. doi: 10.1021/acs.est.3c08209. Epub 2023 Dec 27.
3
Identifying laboratory sources of microplastic and nanoplastic contamination from the air, water, and consumables.
识别来自空气、水和耗材的微塑料和纳米塑料污染的实验室来源。
J Hazard Mater. 2024 Mar 5;465:133276. doi: 10.1016/j.jhazmat.2023.133276. Epub 2023 Dec 16.
4
Long-range atmospheric transport of microplastics across the southern hemisphere.微塑料在南半球的远距离大气传输。
Nat Commun. 2023 Nov 30;14(1):7898. doi: 10.1038/s41467-023-43695-0.
5
Nanoplastics and ultrafine microplastic in the Dutch Wadden Sea - The hidden plastics debris?荷兰瓦登海的纳米塑料和超细微塑料——隐藏的塑料碎片?
Sci Total Environ. 2022 Nov 10;846:157371. doi: 10.1016/j.scitotenv.2022.157371. Epub 2022 Jul 18.
6
Long-range transport of atmospheric microplastics deposited onto glacier in southeast Tibetan Plateau.长距离传输大气微塑料沉积在青藏高原东南部的冰川上。
Environ Pollut. 2022 Aug 1;306:119415. doi: 10.1016/j.envpol.2022.119415. Epub 2022 May 5.
7
Sources and fate of atmospheric microplastics revealed from inverse and dispersion modelling: From global emissions to deposition.大气微塑料的来源和归宿:从全球排放到沉积的反演和弥散模拟。
J Hazard Mater. 2022 Jun 15;432:128585. doi: 10.1016/j.jhazmat.2022.128585. Epub 2022 Feb 26.
8
Nanoplastics measurements in Northern and Southern polar ice.南北极冰中纳米塑料的测量。
Environ Res. 2022 May 15;208:112741. doi: 10.1016/j.envres.2022.112741. Epub 2022 Jan 19.
9
Microplastic pollution in mountain terrains and foothills: A review on source, extraction, and distribution of microplastics in remote areas.山区和山麓的微塑料污染:偏远地区微塑料的来源、提取和分布综述。
Environ Res. 2022 May 1;207:112232. doi: 10.1016/j.envres.2021.112232. Epub 2021 Oct 20.
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Chemical Analysis of Microplastics and Nanoplastics: Challenges, Advanced Methods, and Perspectives.微塑料和纳米塑料的化学分析:挑战、先进方法及展望
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