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长距离传输大气微塑料沉积在青藏高原东南部的冰川上。

Long-range transport of atmospheric microplastics deposited onto glacier in southeast Tibetan Plateau.

机构信息

College of Earth and Environment Sciences, Lanzhou University, Lanzhou, 730000, China.

State Key Laboratory of Cryospheric Science, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou, 730000, China.

出版信息

Environ Pollut. 2022 Aug 1;306:119415. doi: 10.1016/j.envpol.2022.119415. Epub 2022 May 5.

Abstract

Micoroplastics (MPs) can be transported through atmospheric circulations, and have caused global attentions due to their potential risk to the environment. In this study, MPs in snowpit samples collected from Demula (DML) glacier in southeast Tibetan Plateau were investigated. The results showed that the average abundance of MPs in snow was 9.55 ± 0.9 items L, with dominant shapes of plastic fibers and films. MPs size was dominated by MPs <200 μm, with detected minimum size of 48 μm from the DML glacier. MPs in snowpit indicated seasonal variations, showing relatively higher abundance during the monsoon season than that during the non-monsoon season. The chemical composition of MPs and backward air mass trajectory modeling revealed that MPs in DML snowpit mostly originated from the atmospheric long-range transport, suggesting the glacier in southeast Tibetan Plateau can be a temporal sink of atmospheric MPs. The surface structure of the MPs was rough and adhered to a large amount of mineral dust and metallic particles, revealed that these MPs have undergone severe weathering during transportation and after deposition. Based on the MPs data, multi-year average precipitation, and glacier mass balance of DML glacier, the deposition flux of MPs on DML glacier was estimated to be about 7640 ± 720 to 9550 ± 900 items m yr and the export from melting water was about 5.9 ± 1.3 × 10 to 6.6 ± 1.4 × 10 items yr, indicating the glacier may be also an important source of MPs to the downstream ecosystems. These results provided the current status of MPs pollution on the Tibetan Plateau glaciers and new data to the study of MPs in typical cryospheric regions.

摘要

微塑料(MPs)可以通过大气环流传输,由于其对环境的潜在风险,引起了全球关注。本研究调查了青藏高原东南部德木拉(DML)冰川雪坑样品中的 MPs。结果表明,雪样中 MPs 的平均丰度为 9.55±0.9 个 L,主要形态为塑料纤维和薄膜。MPs 尺寸主要集中在 MPs<200μm,在 DML 冰川中检测到的最小尺寸为 48μm。雪坑中的 MPs 存在季节性变化,在季风季节的丰度相对高于非季风季节。MPs 的化学组成和后向轨迹模型表明,DML 雪坑中的 MPs 主要来源于大气长距离传输,表明青藏高原东南部的冰川可能是大气 MPs 的临时汇。MPs 的表面结构粗糙,附着大量矿物灰尘和金属颗粒,表明这些 MPs 在运输和沉积后经历了严重的风化。基于 MPs 数据、DML 冰川多年平均降水量和冰川质量平衡,估算出 DML 冰川上 MPs 的沉积通量约为 7640±720 至 9550±900 个 m yr,融水中的输出通量约为 5.9±1.3×10至 6.6±1.4×10 个 yr,表明冰川也是 MPs 向下游生态系统的重要来源。这些结果提供了青藏高原冰川上 MPs 污染的现状和典型冰冻圈地区 MPs 研究的新数据。

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