Moon Seongphill, Jiang Yuxuan, Neu Jennifer, Siegrist Theo, Ozerov Mykhaylo, Jiang Zhigang, Smirnov Dmitry
National High Magnetic Field Laboratory, Tallahassee, Florida 32310, United States.
Department of Physics, Florida State University, Tallahassee, Florida 32310, United States.
Nano Lett. 2025 Feb 19;25(7):2858-2863. doi: 10.1021/acs.nanolett.4c06072. Epub 2025 Feb 7.
Theories have revealed the universality of the band tilting effect in topological Weyl semimetals (WSMs) and its implications for the material physical properties. However, the experimental identification of tilted Weyl bands remains less explored. Here, we report the magneto-optical evidence of the tilting effect in WSM niobium phosphide. Specifically, we observe Landau level transitions with rich features that are well reproduced within a model of coupled tilted Weyl points. Our analysis indicates that the tilting effect relaxes the selection rules and leads to transitions that would otherwise be forbidden in the non-tilt case. Additionally, we observe unconventional interband transitions with flat and negative magnetic field dispersions, highlighting the importance of coupling between Weyl points. Our results not only emphasize the significance of the tilting effect in the optical responses of WSMs but also demonstrate magneto-optics as an effective tool for probing the tilting effect in electronic band structures.
理论揭示了拓扑外尔半金属(WSMs)中能带倾斜效应的普遍性及其对材料物理性质的影响。然而,倾斜外尔能带的实验识别仍较少被探索。在此,我们报告了WSM磷化铌中倾斜效应的磁光证据。具体而言,我们观察到具有丰富特征的朗道能级跃迁,这些跃迁在耦合倾斜外尔点模型中得到了很好的重现。我们的分析表明,倾斜效应放宽了选择规则,并导致了在非倾斜情况下原本被禁止的跃迁。此外,我们观察到具有平坦和负磁场色散的非常规带间跃迁,突出了外尔点之间耦合的重要性。我们的结果不仅强调了倾斜效应在WSMs光学响应中的重要性,还证明了磁光作为探测电子能带结构中倾斜效应的有效工具。