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用于等离激元学中非局部费贝尔曼参数的计算麦克斯韦求解器

A Computational Maxwell Solver for Nonlocal Feibelman Parameters in Plasmonics.

作者信息

Huber Lorenz, Hohenester Ulrich

机构信息

Institute of Physics, University of Graz, Universitätsplatz 5, 8010 Graz, Austria.

出版信息

J Phys Chem C Nanomater Interfaces. 2025 Jan 23;129(5):2590-2598. doi: 10.1021/acs.jpcc.4c07387. eCollection 2025 Feb 6.

Abstract

Feibelman parameters provide a convenient means to account for quantum surface effects in classical Maxwell descriptions. Recent work has shown that for incoming fields with spatial variations in the nanometer range, for instance those produced by quantum emitters in the vicinity of metallic nanoparticles, nonlocality in the directions parallel to the interface must be considered. Here we develop the methodology for mesoscopic boundary conditions incorporating nonlocal Feibelman parameters, and show how to implement them in a computational Maxwell solver based on the boundary element method. We compare our results with Mie solutions for single and coupled spheres, and find very good agreement throughout.

摘要

费贝尔曼参数为在经典麦克斯韦描述中考虑量子表面效应提供了一种便捷方法。最近的研究表明,对于在纳米范围内具有空间变化的入射场,例如由金属纳米颗粒附近的量子发射器产生的场,必须考虑平行于界面方向的非局域性。在这里,我们开发了包含非局部费贝尔曼参数的介观边界条件的方法,并展示了如何在基于边界元法的计算麦克斯韦求解器中实现这些条件。我们将我们的结果与单球体和耦合球体的米氏解进行比较,发现整体上非常吻合。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7e33/11808787/5d1ada515e99/jp4c07387_0005.jpg

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