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用于制备碳基材料的塑料废弃物:近期在环境可持续性、二氧化碳捕获及绿色能源方面的应用研究

Plastic wastes for carbon-based materials: Investigations on recent applications towards environmentally sustainable, carbon dioxide capture and green energy.

作者信息

Luu The-Anh, Le Van-Giang, Thai Van-Anh, Nguyen Minh-Ky, Lin Chitsan, Pham Minh-Thuan, Chang S Woong, Nguyen D Duc

机构信息

Central Institute for Natural Resources and Environmental Studies, Vietnam National University (CRES-VNU), Hanoi, 111000, Viet Nam.

Ho Chi Minh City Open University, Ho Chi Minh City, 700000, Viet Nam.

出版信息

Environ Pollut. 2025 Apr 1;370:125899. doi: 10.1016/j.envpol.2025.125899. Epub 2025 Feb 20.

Abstract

The rapid growth in plastic production, coupled with inadequate waste management, has led to a significant accumulation of plastic waste in different environments. This raises substantial concerns about long-term ecological impacts, including bioaccumulation in organisms and potential risks to human health. This review focuses on plastic waste-derived carbon materials (PWCMs) and their role in promoting sustainable, eco-friendly energy solutions. The novelty of the study examines the current progress in converting plastic waste into carbon-based materials, with a particular emphasis on recent applications in environmentally sustainable practices, carbon dioxide capture, and green energy solutions. The growing interest in carbon-based materials is due to their unique characteristics, including high specific surface area, porosity, electronic conductivity, stable structure, and versatile surface chemistry. The utilization of PWCMs and their composites has shown promise in absorbing a wide range of contaminants. For organic pollutants, this includes dyes such as methylene blue and pharmaceuticals like antibiotics, polycyclic aromatic hydrocarbons (PAHs), and other endocrine-disrupting chemicals (EDCs). For inorganic contaminants, PWCMs effectively target heavy metals, i.e., cadmium, lead, mercury, and arsenic, as well as anions like nitrate and phosphate. Converting waste plastics into carbonaceous adsorbents holds excellent potential for removing up to 99% of toxic metal elements from wastewater. Furthermore, carbon capture through PWCMs provides an environmentally friendly and practical approach to closing the carbon loop, advancing carbon neutrality, and fostering a more sustainable future. Repurposing waste plastic for hydrogen production has significant potential to contribute to decarbonization efforts and accelerate achieving sustainable development goals (SDGs). The findings also offer valuable insights into the advanced uses of PWCMs, encouraging future efforts in upcycling plastic waste for innovative and sustainable solutions. Yet, a comprehensive evaluation of PWCM applications and their limitations is needed to guide future research toward optimizing their synthesis for economic and environmental sustainability.

摘要

塑料产量的快速增长,加上废物管理不善,导致不同环境中塑料废物大量堆积。这引发了人们对长期生态影响的重大担忧,包括生物体内的生物累积以及对人类健康的潜在风险。本综述聚焦于源自塑料废物的碳材料(PWCMs)及其在促进可持续、环保能源解决方案中的作用。该研究的新颖之处在于审视了将塑料废物转化为碳基材料的当前进展,特别强调了其在环境可持续实践、二氧化碳捕获和绿色能源解决方案中的最新应用。对碳基材料的兴趣日益浓厚,是因为它们具有独特的特性,包括高比表面积、孔隙率、电子导电性、稳定的结构以及多样的表面化学性质。PWCMs及其复合材料的利用在吸收多种污染物方面已展现出前景。对于有机污染物,这包括亚甲基蓝等染料以及抗生素、多环芳烃(PAHs)和其他内分泌干扰化学物质(EDCs)等药物。对于无机污染物,PWCMs能有效针对重金属,即镉、铅、汞和砷,以及硝酸盐和磷酸盐等阴离子。将废塑料转化为碳质吸附剂在从废水中去除高达99%的有毒金属元素方面具有巨大潜力。此外,通过PWCMs进行碳捕获为闭合碳循环、推进碳中和以及培育更可持续的未来提供了一种环境友好且实用的方法。将废塑料重新用于制氢具有巨大潜力,有助于脱碳努力并加速实现可持续发展目标(SDGs)。这些发现还为PWCMs的先进用途提供了有价值的见解,鼓励未来在将塑料废物升级再造以实现创新和可持续解决方案方面做出努力。然而,需要对PWCMs的应用及其局限性进行全面评估,以指导未来研究优化其合成,实现经济和环境的可持续性。

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