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电子掺杂铜酸盐中空穴超导与量子临界反铁磁涨落之间的相互作用

Interplay between hole superconductivity and quantum critical antiferromagnetic fluctuations in electron-doped cuprates.

作者信息

Song Dongjoon, Lee Suheon, Shen Zecheng, Jung Woobin, Lee Wonjun, Choi Sungkyun, Kyung Wonshik, Jung Saegyeol, Cheng Cheng-Maw, Kwon Junyoung, Ishida S, Yoshida Y, Park Seung Ryong, Eisaki H, Wang Yao, Choi Kwang-Yong, Kim C

机构信息

Stewart Blusson Quantum Matter Institute, University of British Columbia, Vancouver, BC, V6T 1Z4, Canada.

Center for Correlated Electron Systems, Institute for Basic Science (IBS), Seoul, 08826, Korea.

出版信息

Nat Commun. 2025 Mar 20;16(1):2764. doi: 10.1038/s41467-025-57942-z.

Abstract

Antiferromagnetic spin fluctuations are the most promising candidate as the pairing glue of high critical temperature (T) superconductivity in cuprates. However, many-body states and intertwined orders have made it difficult to determine how electrons couple with fluctuating spins to form Cooper pairs. Recent experimental and theoretical studies have suggested spin fluctuation-driven quasiparticle band folding, but the relationship between the resultant Fermi pockets and superconductivity remains unclear. Here, using angle-resolved photoemission spectroscopy and numerical simulations, we show a proportional relationship between T and the quasiparticle weight of the incipient hole pocket near the nodal point in electron-doped PrLaCeCuO. Through complementary muon spin spectroscopy measurements, we uncover that the hole pocket forms only in the regime of the fluctuating antiferromagnetic ground state around a presumed quantum critical point. Our observations highlight the significance of the electron-spin fluctuation interaction in enhancing the hole pocket and consequently driving superconductivity.

摘要

反铁磁自旋涨落是铜酸盐中高临界温度(T)超导配对凝聚最有前景的候选者。然而,多体状态和交织序使得确定电子如何与涨落自旋耦合形成库珀对变得困难。最近的实验和理论研究表明了自旋涨落驱动的准粒子能带折叠,但由此产生的费米面口袋与超导之间的关系仍不清楚。在这里,我们使用角分辨光电子能谱和数值模拟,展示了在电子掺杂的PrLaCeCuO中,T与节点附近初始空穴口袋的准粒子权重之间的比例关系。通过互补的μ子自旋谱测量,我们发现空穴口袋仅在围绕假定量子临界点的反铁磁涨落基态区域形成。我们的观察突出了电子 - 自旋涨落相互作用在增强空穴口袋并进而驱动超导方面的重要性。

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