Zhong Yu-Jie, Li Jia-Cheng, Huang Xuan-Fu, Lee Ying-Je, Chen Ting-Zhen, Zhang Jia-Ren, Huang Angus, Hsu Hsiu-Chuan, Ortix Carmine, Chang Ching-Hao
Department of Physics, National Cheng Kung University, Tainan 70101, Taiwan.
Center for Quantum Frontiers of Research and Technology (QFort), National Cheng Kung University, Tainan 70101, Taiwan.
Nano Lett. 2025 Apr 9;25(14):5550-5556. doi: 10.1021/acs.nanolett.4c03694. Epub 2025 Mar 28.
We theoretically demonstrate that carbon nanoscrolls, spirally wrapped graphene layers with open end points, can be characterized by a large positive magnetoconductance. We show that when a carbon nanoscroll is subject to an axial magnetic field of several Tesla, the ballistic conductance at low carrier densities of the nanoscroll increases by about 200%. Importantly, we find that this positive magnetoconductance is not only preserved in an imperfect nanoscroll (with disorder or mild interturn misalignment) but can even be enhanced in the presence of on-site disorder. We prove that the positive magnetoconductance comes about with the emergence of magnetic-field-induced zero-energy modes, specific to rolled-up geometries. Our results establish curved graphene systems as a new material platform displaying sizable magnetoresistive phenomena.
我们从理论上证明,具有开放端点的螺旋缠绕石墨烯层——碳纳米卷,可表现出显著的正磁电导特性。我们发现,当碳纳米卷处于几特斯拉的轴向磁场中时,在低载流子密度下,纳米卷的弹道电导会增加约200%。重要的是,我们发现这种正磁电导不仅在不完美的碳纳米卷(存在无序或轻微的匝间错位)中得以保留,甚至在存在局域无序的情况下还会增强。我们证明,正磁电导是由磁场诱导的零能量模式的出现所导致的,这是卷曲几何结构所特有的。我们的研究结果确立了弯曲石墨烯系统作为一种展现出可观磁阻现象的新型材料平台。