Wu Shuhan, Xu Zijian, Li Ruoru, Chen Sheng, Zhang Yingling, Zhang Xiangzhi, Chen Zhenhua, Tai Renzhong
Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800, China.
Shanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201204, China.
Nanomaterials (Basel). 2025 Mar 26;15(7):496. doi: 10.3390/nano15070496.
Scanning transmission X-ray microscopy (STXM) is a direct imaging technique with nanoscale resolution. But its resolution is limited by the spot size on the sample, i.e., by the manufacturing technique of the focusing element. As an emerging high-resolution X-ray imaging technique, ptychography utilizes highly redundant data from overlapping scans as well as phase retrieval algorithms to simultaneously reconstruct a high-resolution sample image and a probe function. In this study, we designed an accurate reconstruction strategy to obtain the probe spot with the vibration effects being eliminated, and developed an image enhancement technique for STXM by combining the reconstructed probe with the deconvolution algorithm. This approach significantly improves the resolution of STXM imaging and can break the limitation of the focal spot on STXM resolution when the scanning step size is near or below the spot size, while the data processing time is much shorter than that of ptychography. Both simulations and experiments show that this approach can be applied to STXM data at different energies and different scan steps using the same focal spot retrieved via ptychography.
扫描透射X射线显微镜(STXM)是一种具有纳米级分辨率的直接成像技术。但其分辨率受样品上光斑尺寸的限制,即受聚焦元件制造技术的限制。作为一种新兴的高分辨率X射线成像技术,叠层成像利用来自重叠扫描的高度冗余数据以及相位恢复算法来同时重建高分辨率的样品图像和探针函数。在本研究中,我们设计了一种精确的重建策略以在消除振动影响的情况下获得探针光斑,并通过将重建的探针与去卷积算法相结合,开发了一种用于STXM的图像增强技术。这种方法显著提高了STXM成像的分辨率,并且当扫描步长接近或低于光斑尺寸时,可以突破焦斑对STXM分辨率的限制,同时数据处理时间比叠层成像短得多。模拟和实验均表明,该方法可应用于使用通过叠层成像获取的相同焦斑的不同能量和不同扫描步长的STXM数据。