Yao Yudong, Jiang Yi, Klug Jeffrey, Nashed Youssef, Roehrig Christian, Preissner Curt, Marin Fabricio, Wojcik Michael, Cossairt Oliver, Cai Zhonghou, Vogt Stefan, Lai Barry, Deng Junjing
Advanced Photon Source, Argonne National Laboratory, IL 60439, USA.
Mathematics and Computer Science Division, Argonne National Laboratory, IL 60439, USA.
J Synchrotron Radiat. 2021 Jan 1;28(Pt 1):309-317. doi: 10.1107/S1600577520014708.
Ptychography is a rapidly developing scanning microscopy which is able to view the internal structures of samples at a high resolution beyond the illumination size. The achieved spatial resolution is theoretically dose-limited. A broadband source can provide much higher flux compared with a monochromatic source; however, it conflicts with the necessary coherence requirements of this coherent diffraction imaging technique. In this paper, a multi-wavelength reconstruction algorithm has been developed to deal with the broad bandwidth in ptychography. Compared with the latest development of mixed-state reconstruction approach, this multi-wavelength approach is more accurate in the physical model, and also considers the spot size variation as a function of energy due to the chromatic focusing optics. Therefore, this method has been proved in both simulation and experiment to significantly improve the reconstruction when the source bandwidth, illumination size and scan step size increase. It is worth mentioning that the accurate and detailed information of the energy spectrum for the incident beam is not required in advance for the proposed method. Further, we combine multi-wavelength and mixed-state approaches to jointly solve temporal and spatial partial coherence in ptychography so that it can handle various disadvantageous experimental effects. The significant relaxation in coherence requirements by our approaches allows the use of high-flux broadband X-ray sources for high-efficient and high-resolution ptychographic imaging.
叠层成像术是一种快速发展的扫描显微镜技术,它能够以高于照明尺寸的高分辨率观察样品的内部结构。所实现的空间分辨率在理论上受剂量限制。与单色光源相比,宽带光源可以提供更高的通量;然而,这与这种相干衍射成像技术所需的相干性要求相冲突。在本文中,已开发出一种多波长重建算法来处理叠层成像术中的宽带宽问题。与混合态重建方法的最新进展相比,这种多波长方法在物理模型上更准确,并且还考虑了由于色差聚焦光学元件导致的光斑尺寸随能量的变化。因此,在模拟和实验中均已证明,当光源带宽、照明尺寸和扫描步长增加时,该方法能显著改善重建效果。值得一提的是,所提出的方法无需预先获得入射光束能谱的准确详细信息。此外,我们将多波长方法和混合态方法相结合,共同解决叠层成像术中的时间和空间部分相干性问题,以便它能够处理各种不利的实验效应。我们的方法对相干性要求的显著放宽使得能够使用高通量宽带X射线源进行高效高分辨率的叠层成像。