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铬电子能带中自旋和电荷密度波的证据。

Evidence of spin and charge density waves in Chromium electronic bands.

作者信息

Bisti Federico, Settembri Paolo, Minár Jan, Rogalev Victor A, Widmer Roland, Gröning Oliver, Shi Ming, Schmitt Thorsten, Profeta Gianni, Strocov Vladimir N

机构信息

Dipartimento di Scienze Fisiche e Chimiche, Università dell'Aquila, L'Aquila, Italy.

Swiss Light Source, Paul Scherrer Institute, Villigen, PSI Switzerland.

出版信息

Commun Mater. 2025;6(1):70. doi: 10.1038/s43246-025-00789-0. Epub 2025 Apr 12.

Abstract

The incommensurate spin density wave (SDW) of Chromium represents the classic example of itinerant antiferromagnetism induced by the nesting of the Fermi surface, which is further enriched by the co-presence of a charge density wave (CDW). Here, we explore its electronic band structure using soft-X-ray angle-resolved photoemission spectroscopy (ARPES) for a proper bulk-sensitive investigation. We find that the long-range magnetic order gives rise to a very rich ARPES signal, which can only be interpreted with a proper first-principles description of the SDW and CDW, combined with a band unfolding procedure, reaching a remarkable agreement with experiments. Additional features of the SDW order are obscured by superimposed effects related to the photoemission process, which, unexpectedly, are not predicted by the free-electron model for the final states. We demonstrate that, even for excitation photon energies up to 1 keV, a multiple scattering description of the photoemission final states is required.

摘要

铬的非公度自旋密度波(SDW)是由费米面嵌套诱导的巡游反铁磁性的经典例子,电荷密度波(CDW)的共存进一步丰富了这一现象。在此,我们使用软X射线角分辨光电子能谱(ARPES)来研究其电子能带结构,以进行适当的体敏感研究。我们发现,长程磁序产生了非常丰富的ARPES信号,这只能通过对SDW和CDW进行适当的第一性原理描述,并结合能带展开程序来解释,从而与实验达成显著一致。SDW序的其他特征被与光发射过程相关的叠加效应所掩盖,而这些效应出乎意料地未被终态的自由电子模型所预测。我们证明,即使对于高达1 keV的激发光子能量,也需要对光发射终态进行多重散射描述。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7126/11993358/97e1e3b23869/43246_2025_789_Fig1_HTML.jpg

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