Patterson Andrew, Boyle Nina, John Josh, Wang Mingxun, Mannochio-Russo Helena, Pyo Jeong Joo, Kim Min Soo, Tian Shuchang, Koo Imhoi, Anitha Mallappa, Tian Yuan, Morgan Ethan, Murray Iain, Perdew Gary, Wu Gary, Dorrestein Pieter, Bisanz Jordan, Redinbo Matthew
Pennsylvania State University.
Penn State University.
Res Sq. 2025 Apr 8:rs.3.rs-6321321. doi: 10.21203/rs.3.rs-6321321/v1.
Glucuronidation is an important detoxification pathway that operates in balance with gastrointestinal microbial β-glucuronidase (GUS) enzymes that can regenerate active metabolites from their glucuronidated forms. Although significant progress has been made in characterizing GUS enzymes, methods to comprehensively define the glucuronidome - the collection of glucuronidated metabolites - remain limited. In this study we employed pattern-filtering data science approaches alongside untargeted LC-MS/MS metabolomics to map the glucuronidome in urine, serum, and colon/fecal samples from gnotobiotic and conventional mice. Our findings reveal microbiome-driven shifts in the glucuronidome, highlighting how differential GUS activity can influence host metabolite profiles. Reverse metabolomics of known glucuronidated chemicals and glucuronidation pattern filtering searches in public metabolomics datasets exposed the diversity of glucuronidated metabolites in human and mouse ecosystems. In summary, we present a new glucuronidation fingerprint resource that provides broader access to and analysis of the glucuronidome. By systematically capturing glucuronidation patterns, this resource enhances unknown metabolite annotation efforts and provides new insights into the dynamic relationship between the host and bacterial biotransformation activities.
葡萄糖醛酸化是一条重要的解毒途径,它与胃肠道微生物β-葡萄糖醛酸酶(GUS)保持平衡,GUS酶能够将葡萄糖醛酸化形式的活性代谢物再生出来。尽管在表征GUS酶方面已取得显著进展,但全面定义葡萄糖醛酸化代谢组(即葡萄糖醛酸化代谢物的集合)的方法仍然有限。在本研究中,我们采用模式过滤数据科学方法并结合非靶向液相色谱-串联质谱代谢组学技术,来绘制悉生小鼠和常规小鼠尿液、血清以及结肠/粪便样本中的葡萄糖醛酸化代谢组图谱。我们的研究结果揭示了微生物群驱动的葡萄糖醛酸化代谢组变化,突出了不同的GUS活性如何影响宿主代谢物谱。对已知葡萄糖醛酸化化学物质的反向代谢组学分析以及在公共代谢组学数据集中进行的葡萄糖醛酸化模式过滤搜索,揭示了人类和小鼠生态系统中葡萄糖醛酸化代谢物的多样性。总之,我们提供了一种新的葡萄糖醛酸化指纹资源,可更广泛地获取和分析葡萄糖醛酸化代谢组。通过系统地捕捉葡萄糖醛酸化模式,该资源加强了未知代谢物的注释工作,并为宿主与细菌生物转化活性之间的动态关系提供了新的见解。