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利用音叉谐振器探测 Kagome 金属 CsVSb 的轨道磁性

Probing orbital magnetism of a kagome metal CsVSb by a tuning fork resonator.

作者信息

Gui Hengrui, Yang Lin, Wang Xiaoyu, Chen Dong, Shi Zekai, Zhang Jiawen, Wei Jia, Zhou Keyi, Schnelle Walter, Zhang Yongjun, Liu Yu, Bangura Alimamy F, Wang Ziqiang, Felser Claudia, Yuan Huiqiu, Jiao Lin

机构信息

Center for Correlated Matter and School of Physics, Zhejiang University, Hangzhou, China.

College of Materials and Environmental Engineering, Hangzhou Dianzi University, Hangzhou, China.

出版信息

Nat Commun. 2025 May 8;16(1):4275. doi: 10.1038/s41467-025-59534-3.

Abstract

The recently discovered kagome metal CsVSb exhibits a complex phase diagram that encompasses frustrated magnetism, topological charge density wave (CDW), and superconductivity. One CDW state that breaks time-reversal symmetry was proposed in this compound, while the exact nature of the putative magnetic state remains elusive. To examine the thermodynamic state of CsVSb and assess the character of the associated magnetism, we conducted tuning fork resonator measurements of magnetotropic susceptibility over a broad range of angles, magnetic fields, and temperatures. We found a cascade of phase transitions in the CDW phase. Of particular interest is a highly anisotropic magnetic structure that arises below about 30 K, with a magnetic moment along the c-axis that has an extremely small magnitude. This magnetic state demonstrates extremely slow dynamics and small saturate field, all suggest that electronic phase below 30 K breaks time reversal symmetry and has an unconventional origin.

摘要

最近发现的 Kagome 金属 CsVSb 展现出一个复杂的相图,其中包含受挫磁性、拓扑电荷密度波(CDW)和超导性。在这种化合物中提出了一种打破时间反演对称性的 CDW 态,而假定磁态的确切性质仍然难以捉摸。为了研究 CsVSb 的热力学状态并评估相关磁性的特征,我们在广泛的角度、磁场和温度范围内进行了磁致磁化率的音叉谐振器测量。我们在 CDW 相中发现了一系列相变。特别有趣的是,在约 30 K 以下出现了一种高度各向异性的磁性结构,其沿 c 轴的磁矩大小极小。这种磁态表现出极其缓慢的动力学和小的饱和场,所有这些都表明 30 K 以下的电子相打破了时间反演对称性且具有非常规起源。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f796/12062287/e30f8d99a6eb/41467_2025_59534_Fig1_HTML.jpg

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