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压力诱导的AgSnSe态密度再分布及超导性的重现

Pressure-induced redistribution in density of states and reemergence of superconductivity in AgSnSe.

作者信息

Pei Cuiying, Wu Juefei, Cao Weizheng, Jiang Yuyang, Wang Qi, Zhao Yi, Wang Junjie, Ying Tianping, Qi Yanpeng

机构信息

School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China.

ShanghaiTech Laboratory for Topological Physics, ShanghaiTech University, Shanghai 201210, China.

出版信息

iScience. 2025 Apr 15;28(5):112442. doi: 10.1016/j.isci.2025.112442. eCollection 2025 May 16.

Abstract

The intricate relationship between superconductivity and disorder is a captivating subject within condensed matter physics. Strong disorder suppresses superconductivity and induces a superconductor-insulator transition. However, below a certain critical degree of disorder, the superconductivity critical temperature ( ) can be enhanced. Herein, we present evidence of pressure-induced reemergence of superconductivity in a strongly disordered 3D superconductor AgSnSe. A structural phase transition from NaCl- to CsCl-type structure occurs, coinciding with the emergence of the second superconducting state. First-principles calculations suggest that the partial density of states in Se atoms exhibits a sharp elevation around the transition pressure, which is related to the secondary superconducting state. Our study illustrates AgSnSe as a promising platform to explore the comprehensive effects among disorder, high pressure, and superconductivity, offering insights for subsequent experimental and theoretical studies.

摘要

超导性与无序之间的复杂关系是凝聚态物理中一个引人入胜的课题。强无序会抑制超导性并引发超导体-绝缘体转变。然而,在低于某个特定的无序临界程度时,超导临界温度( )会增强。在此,我们展示了在强无序三维超导体AgSnSe中压力诱导超导性重新出现的证据。发生了从NaCl型到CsCl型结构的结构相变,这与第二个超导态的出现相吻合。第一性原理计算表明,Se原子的部分态密度在转变压力附近呈现出急剧升高,这与次级超导态有关。我们的研究表明AgSnSe是探索无序、高压和超导性之间综合效应的一个有前景的平台,为后续的实验和理论研究提供了见解。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/eb53/12059703/71c24df056af/fx1.jpg

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