Oladejo Olubusayo F, Olukotun Stephen F, Rufai Abdulfatai B, Mathuthu Manny
Department of Physics, Osun State University, Osogbo, Nigeria.
Department of Physics and Engineering Physics, Obafemi Awolowo University, Ile-Ife, Nigeria.
Sci Rep. 2025 Jun 2;15(1):19345. doi: 10.1038/s41598-025-02239-w.
This study assessed the radioactivity levels of naturally occurring radioactive materials (NORMs), specifically K, Th, and U, in quarry products and surrounding soils from four major commercial quarry sites in Osun State, Nigeria, using gamma spectroscopic technique. The average activity concentrations of K, Th, and U in the quarry products are 332.55 ± 28.8, 9.72 ± 1.0, and 11.35 ± 1.0 Bq/kg, respectively, all below global averages. Radiation risk indices, including radium equivalent levels, effective dose rates, absorbed dose rates, gamma radioactivity level index, internal and external hazard indices, and gonadal dose equivalent, were evaluated. The radium equivalent levels ranged from 48.77 to 53.25 Bq/kg, well below the global limit of 370 Bq/kg, while the absorbed dose rates were 40% lower than the global average. Total effective dose rates and hazard indices were also significantly below safety thresholds, indicating negligible radiation threats. Statistical analysis revealed strong correlations between K and radiological indices, showing its dominant influence on overall radiation risk. Correlation and hierarchical cluster analysis further affirmed that the evaluated radiological risks were dependent on the radionuclides measured concentrations. The results conclude that both the quarry products and surrounding soils pose no significant radiation hazards, rendering them safe for construction and human activities.
本研究采用伽马能谱技术,评估了尼日利亚奥孙州四个主要商业采石场的采石产品及周边土壤中天然存在的放射性物质(NORMs),特别是钾(K)、钍(Th)和铀(U)的放射性水平。采石产品中K、Th和U的平均活度浓度分别为332.55±28.8、9.72±1.0和11.35±1.0 Bq/kg,均低于全球平均水平。评估了镭当量水平、有效剂量率、吸收剂量率、伽马放射性水平指数、内外照射危害指数以及性腺剂量当量等辐射风险指标。镭当量水平在48.77至53.25 Bq/kg之间,远低于370 Bq/kg的全球限值,而吸收剂量率比全球平均水平低40%。总有效剂量率和危害指数也显著低于安全阈值,表明辐射威胁可忽略不计。统计分析表明K与放射学指标之间存在强相关性,显示出其对总体辐射风险的主导影响。相关性和层次聚类分析进一步证实,评估的放射学风险取决于所测放射性核素的浓度。结果表明,采石产品和周边土壤均不存在显著的辐射危害,使其对建筑和人类活动而言是安全的。