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通过耦合谐振子模型对超强光与物质相互作用的描述及其与腔量子电动力学哈密顿量的联系。

Description of ultrastrong light-matter interaction through coupled harmonic oscillator models and their connection with cavity-QED Hamiltonians.

作者信息

Muniain Unai, Aizpurua Javier, Hillenbrand Rainer, Martín-Moreno Luis, Esteban Ruben

机构信息

Donostia International Physics Center, Paseo Manuel de Lardizabal 4, 20018 Donostia-San Sebastián, Spain.

IKERBASQUE, Basque Foundation for Science, María Díaz de Haro 3, 48013 Bilbao, Spain.

出版信息

Nanophotonics. 2025 Mar 11;14(11):2031-2052. doi: 10.1515/nanoph-2024-0528. eCollection 2025 Jun.

Abstract

Classical coupled harmonic oscillator models are capable of describing the optical and infrared response of nanophotonic systems where a cavity photon couples to dipolar matter excitations. The distinct forms of coupling adopted in these classical models lead to different results in the ultrastrong coupling regime. To clarify the specific classical model required to address particular configurations, we establish a connection between each oscillator model and the equivalent cavity Quantum Electrodynamics description. We show that the proper choice of coupled harmonic oscillator model depends on the presence or absence of the diamagnetic term in the quantum models, linked to whether transverse or longitudinal electromagnetic fields mediate the coupling. This analysis also shows how to exploit the classical oscillator models to extract measurable information of the optical response, as demonstrated in three canonical photonic systems, and to describe the opening of the Reststrahlen band in the bulk dispersion of phononic materials.

摘要

经典耦合谐振子模型能够描述纳米光子系统的光学和红外响应,其中腔光子与偶极物质激发相互耦合。这些经典模型中采用的不同耦合形式在超强耦合 regime 中会导致不同的结果。为了阐明处理特定构型所需的具体经典模型,我们在每个振子模型与等效腔量子电动力学描述之间建立了联系。我们表明,耦合谐振子模型的正确选择取决于量子模型中抗磁项的有无,这与横向或纵向电磁场是否介导耦合有关。该分析还展示了如何利用经典振子模型提取光学响应的可测量信息,如在三个典型光子系统中所证明的那样,以及描述声子材料体色散中 Reststrahlen 带的开启。

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