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垂直堆叠的单片钙钛矿彩色光电探测器。

Vertically stacked monolithic perovskite colour photodetectors.

作者信息

Tsarev Sergey, Proniakova Daria, Liu Xuqi, Wu Erfu, Matt Gebhard J, Sakhatskyi Kostiantyn, Ferraresi Lorenzo L A, Kothandaraman Radha, Fu Fan, Shorubalko Ivan, Yakunin Sergii, Kovalenko Maksym V

机构信息

Laboratory of Inorganic Chemistry, Department of Chemistry and Applied Biosciences, ETH Zürich, Zurich, Switzerland.

Laboratory for Thin Films and Photovoltaics, Empa - Swiss Federal Laboratories for Materials Science and Technology, Dubendorf, Switzerland.

出版信息

Nature. 2025 Jun;642(8068):592-598. doi: 10.1038/s41586-025-09062-3. Epub 2025 Jun 18.

DOI:10.1038/s41586-025-09062-3
PMID:40533540
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12176651/
Abstract

Modern colour image sensors face challenges in further improving sensitivity and image quality because of inherent limitations in light utilization efficiency. A major factor contributing to these limitations is the use of passive optical filters, which absorb and dissipate a substantial amount of light, thereby reducing the efficiency of light capture. On the contrary, active optical filtering in Foveon-type vertically stacked architectures still struggles to deliver optimal performance owing to their lack of colour selectivity, making them inefficient for precise colour imaging. Here we introduce an innovative architecture for colour sensor arrays that uses multilayer monolithically stacked lead halide perovskite thin-film photodetectors. Perovskite bandgap tunability is utilized to selectively absorb the visible light spectrum's red, green and blue regions, eliminating the need for colour filters. External quantum efficiencies of 50%, 47% and 53% are demonstrated for the red, green and blue channels, respectively, as well as a colour accuracy of 3.8% in ΔE outperforming the state-of-the-art colour-filter array and Foveon-type photosensors. The image sensor design improves light utilization in colour sensors and paves the way for the next generation of highly sensitive, artefact-free images with enhanced colour fidelity.

摘要

由于光利用效率的固有局限性,现代彩色图像传感器在进一步提高灵敏度和图像质量上面临挑战。造成这些局限性的一个主要因素是使用了无源光学滤波器,它会吸收并耗散大量光线,从而降低光捕获效率。相反,在Foveon型垂直堆叠架构中的有源光学滤波由于缺乏颜色选择性,仍难以实现最佳性能,使其在精确彩色成像方面效率低下。在此,我们介绍一种用于彩色传感器阵列的创新架构,该架构使用多层单片堆叠的卤化铅钙钛矿薄膜光电探测器。利用钙钛矿的带隙可调性来选择性吸收可见光谱的红、绿、蓝区域,从而无需使用滤色器。红色、绿色和蓝色通道的外量子效率分别达到了50%、47%和53%,并且在ΔE方面的颜色精度为3.8%,优于目前最先进的滤色器阵列和Foveon型光电传感器。这种图像传感器设计提高了彩色传感器中的光利用率,并为下一代具有更高颜色保真度的高灵敏度、无伪像图像铺平了道路。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/bc4a26d20d2a/41586_2025_9062_Fig9_ESM.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/86dfffbfb234/41586_2025_9062_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/13a18934d4e1/41586_2025_9062_Fig5_ESM.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/d0b0594e7a13/41586_2025_9062_Fig6_ESM.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/44f54107ddc4/41586_2025_9062_Fig7_ESM.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/b49b4723cfd0/41586_2025_9062_Fig8_ESM.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/bc4a26d20d2a/41586_2025_9062_Fig9_ESM.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/7ae17b2d15b7/41586_2025_9062_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/0c4359ef1158/41586_2025_9062_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/7c6a8e58d7ed/41586_2025_9062_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/86dfffbfb234/41586_2025_9062_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/13a18934d4e1/41586_2025_9062_Fig5_ESM.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/d0b0594e7a13/41586_2025_9062_Fig6_ESM.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/44f54107ddc4/41586_2025_9062_Fig7_ESM.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/b49b4723cfd0/41586_2025_9062_Fig8_ESM.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a10d/12176651/bc4a26d20d2a/41586_2025_9062_Fig9_ESM.jpg

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本文引用的文献

1
Flexible Stacked Perovskite Photodetectors for High-Efficiency Multicolor Fluorescence Detection.
ACS Appl Mater Interfaces. 2023 Aug 30;15(34):40799-40808. doi: 10.1021/acsami.3c06793. Epub 2023 Aug 16.
2
A Review of Perovskite-Based Photodetectors and Their Applications.基于钙钛矿的光电探测器及其应用综述。
Nanomaterials (Basel). 2022 Dec 9;12(24):4390. doi: 10.3390/nano12244390.
3
Beyond Tristimulus Color Vision with Perovskite-Based Multispectral Sensors.基于钙钛矿的多光谱传感器实现超越三色视觉的彩色视觉。
ACS Appl Mater Interfaces. 2022 Mar 9;14(9):11645-11653. doi: 10.1021/acsami.1c25095. Epub 2022 Feb 22.
4
Monolithic integration of visible GaAs and near-infrared InGaAs for multicolor photodetectors by using high-throughput epitaxial lift-off toward high-resolution imaging systems.通过高通量外延剥离技术实现用于高分辨率成像系统的多色光电探测器的可见 GaAs 和近红外 InGaAs 的单片集成。
Sci Rep. 2019 Dec 9;9(1):18661. doi: 10.1038/s41598-019-55159-x.
5
All-inorganic perovskite nanocrystal scintillators.全无机钙钛矿纳米晶闪烁体。
Nature. 2018 Sep;561(7721):88-93. doi: 10.1038/s41586-018-0451-1. Epub 2018 Aug 27.
6
Charge carrier mobility of disordered organic semiconductors with correlated energetic and spatial disorder.具有相关能量和空间无序的无序有机半导体中的电荷载流子迁移率。
Phys Chem Chem Phys. 2018 Mar 28;20(13):8897-8908. doi: 10.1039/C8CP00544C.
7
Thin single crystal perovskite solar cells to harvest below-bandgap light absorption.用于收获带隙下光吸收的薄单晶钙钛矿太阳能电池。
Nat Commun. 2017 Dec 1;8(1):1890. doi: 10.1038/s41467-017-02039-5.
8
Selective dissolution of halide perovskites as a step towards recycling solar cells.卤化物钙钛矿的选择性溶解,迈向回收太阳能电池的一步。
Nat Commun. 2016 May 23;7:11735. doi: 10.1038/ncomms11735.
9
Organic Photodiodes: The Future of Full Color Detection and Image Sensing.有机光电二极管:全色检测和图像感应的未来。
Adv Mater. 2016 Jun;28(24):4766-802. doi: 10.1002/adma.201505405. Epub 2016 Apr 25.
10
Organic-Inorganic Perovskites: Structural Versatility for Functional Materials Design.有机-无机钙钛矿:功能材料设计的结构多样性。
Chem Rev. 2016 Apr 13;116(7):4558-96. doi: 10.1021/acs.chemrev.5b00715. Epub 2016 Apr 4.