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基于全内反射的用于室温全光开关的钙钛矿微线的微流体辅助生长

Microfluidic-Assisted Growth of Perovskite Microwires for Room-Temperature All-Optical Switching Based on Total Internal Reflection.

作者信息

Coriolano Annalisa, Fieramosca Antonio, Polimeno Laura, Mastria Rosanna, Todisco Francesco, De Giorgi Milena, De Marco Luisa, Rizzo Aurora, Ballarini Dario, Viola Ilenia, Sanvitto Daniele

机构信息

CNR NANOTEC, Institute of Nanotechnology, via Monteroni, 73100 Lecce, Italy.

CNR NANOTEC, Institute of Nanotechnology, c/o Dipt. di Fisica, Sapienza Università, P.le A. Moro 2, I-00185 Rome, Italy.

出版信息

Nano Lett. 2025 Jul 9;25(27):10794-10801. doi: 10.1021/acs.nanolett.5c01866. Epub 2025 Jun 25.

Abstract

The development of efficient integrated photonic circuits is fundamental for ongoing research in information processing and computer science. The greatest challenge facing photonic systems is achieving strong nonlinearities, which are exploitable in strongly coupled systems, leading to the formation of exciton-polaritons. In this context, the use of hybrid organic-inorganic perovskites (PVKs) offers a promising alternative, exhibiting robust interactions at Room Temperature (RT). However, the development of PVK-based integrated devices requires both the ability to achieve long in-plane propagation and the development of alternative fabrication approaches tailored to PVK materials, designed to preserve their optical properties and prevent degradation. Herein, we present the realization of a proof-of-concept all-optical switch using propagating polaritons confined in Total Internal Reflection (TIR), which ensures long in-plane propagation and limited optical losses. We realized efficient injection-extraction of the TIR-confined waveguide polariton modes by employing gold grating couplers prepatterned on the substrate.

摘要

高效集成光子电路的发展是信息处理和计算机科学领域正在进行的研究的基础。光子系统面临的最大挑战是实现强非线性,这在强耦合系统中是可利用的,从而导致激子极化激元的形成。在这种情况下,使用有机-无机杂化钙钛矿(PVK)提供了一种有前途的替代方案,在室温(RT)下表现出强大的相互作用。然而,基于PVK的集成器件的开发既需要实现长平面内传播的能力,也需要开发适合PVK材料的替代制造方法,旨在保留其光学特性并防止降解。在此,我们展示了一种使用全内反射(TIR)中受限的传播极化激元实现的概念验证全光开关,它确保了长平面内传播和有限的光学损耗。我们通过在衬底上预先图案化的金光栅耦合器实现了TIR受限波导极化激元模式的高效注入-提取。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/60d3/12257638/d70a3f40098a/nl5c01866_0001.jpg

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