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钙钛矿极化激元激光器的电极化切换

Electrical polarization switching of perovskite polariton laser.

作者信息

Łempicka-Mirek Karolina, Król Mateusz, De Marco Luisa, Coriolano Annalisa, Polimeno Laura, Viola Ilenia, Kędziora Mateusz, Muszyński Marcin, Morawiak Przemysław, Mazur Rafał, Kula Przemysław, Piecek Wiktor, Fita Piotr, Sanvitto Daniele, Szczytko Jacek, Piętka Barbara

机构信息

Faculty of Physics, Institute of Experimental Physics, University of Warsaw, ul. Pasteura 5, PL-02-093 Warsaw, Poland.

CNR NANOTEC, Institute of Nanotechnology, Via Monteroni, 73100 Lecce, Italy.

出版信息

Nanophotonics. 2024 Feb 19;13(14):2659-2668. doi: 10.1515/nanoph-2023-0829. eCollection 2024 Jun.

Abstract

Optoelectronic and spinoptronic technologies benefit from flexible and tunable coherent light sources combining the best properties of nano- and material-engineering to achieve favorable properties such as chiral lasing and low threshold nonlinearities. In this work we demonstrate an electrically wavelength- and polarization-tunable room temperature polariton laser due to emerging photonic spin-orbit coupling. For this purpose, we design an optical cavity filled with both birefringent nematic liquid crystal and an inorganic perovskite. Our versatile growth method of single CsPbBr inorganic perovskite crystals in polymer templates allows us to reach strong light-matter coupling and pump-induced condensation of exciton-polaritons resulting in coherent emission of light. The sensitivity of the liquid crystal to external voltage permits electrical tuning of the condensate energy across 7 nm; its threshold power, allowing us to electrically switch it on and off; and its state of polarization sweeping from linear to locally tilted circularly polarized emission.

摘要

光电和自旋光电子技术受益于灵活且可调谐的相干光源,这些光源结合了纳米和材料工程的最佳特性,以实现诸如手性激光和低阈值非线性等良好特性。在这项工作中,我们展示了一种由于新兴的光子自旋轨道耦合而实现的电波长和偏振可调的室温极化激元激光器。为此,我们设计了一个充满双折射向列型液晶和无机钙钛矿的光学腔。我们在聚合物模板中生长单 CsPbBr 无机钙钛矿晶体的通用方法使我们能够实现强光 - 物质耦合以及泵浦诱导的激子极化激元凝聚,从而产生相干光发射。液晶对外部电压的敏感性允许对凝聚能进行 7 纳米的电调谐;其阈值功率使我们能够对其进行电开关;并且其偏振状态从线性扫描到局部倾斜的圆偏振发射。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ee22/11636435/41d8b88e9157/j_nanoph-2023-0829_fig_001.jpg

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