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用于室温激子极化激元凝聚和边缘激光发射的预设计钙钛矿晶体波导。

Predesigned perovskite crystal waveguides for room-temperature exciton-polariton condensation and edge lasing.

作者信息

Kędziora Mateusz, Opala Andrzej, Mastria Rosanna, De Marco Luisa, Król Mateusz, Łempicka-Mirek Karolina, Tyszka Krzysztof, Ekielski Marek, Guziewicz Marek, Bogdanowicz Karolina, Szerling Anna, Sigurðsson Helgi, Czyszanowski Tomasz, Szczytko Jacek, Matuszewski Michał, Sanvitto Daniele, Piętka Barbara

机构信息

Institute of Experimental Physics, Faculty of Physics, University of Warsaw, Warsaw, Poland.

Institute of Physics, Polish Academy of Sciences, Warsaw, Poland.

出版信息

Nat Mater. 2024 Nov;23(11):1515-1522. doi: 10.1038/s41563-024-01980-3. Epub 2024 Aug 19.

Abstract

Perovskite crystals-with their exceptional nonlinear optical properties, lasing and waveguiding capabilities-offer a promising platform for integrated photonic circuitry within the strong-coupling regime at room temperature. Here we demonstrate a versatile template-assisted method to efficiently fabricate large-scale waveguiding perovskite crystals of arbitrarily predefined geometry such as microwires, couplers and splitters. We non-resonantly stimulate a condensate of waveguided exciton-polaritons resulting in bright polariton lasing from the transverse interfaces and corners of our perovskite microstructures. Large blueshifts with excitation power and high mutual coherence between the different edge and corner lasing signals are detected in the far-field photoluminescence, implying that a spatially extended condensates of coherent polaritons has formed. The condensate polaritons are found to propagate over long distances in the wires from the excitation spot and can couple to neighbouring wires through large air gaps, making our platform promising for integrated polaritonic circuitry and on-chip optical devices with strong nonlinearities.

摘要

钙钛矿晶体凭借其卓越的非线性光学特性、激光发射和波导能力,为室温下强耦合 regime 内的集成光子电路提供了一个有前景的平台。在此,我们展示了一种通用的模板辅助方法,可高效制造具有任意预定义几何形状(如微线、耦合器和分离器)的大规模波导钙钛矿晶体。我们非共振地激发波导激子 - 极化子凝聚体,导致从我们的钙钛矿微结构的横向界面和角落发出明亮的极化子激光。在远场光致发光中检测到随着激发功率的大幅蓝移以及不同边缘和角落激光信号之间的高相互相干性,这意味着已形成了空间扩展的相干极化子凝聚体。发现凝聚极化子在从激发点开始的微线中能长距离传播,并且可以通过大的气隙耦合到相邻微线,这使得我们的平台有望用于具有强非线性的集成极化子电路和片上光学器件。

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