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解析磁性 Kagome 金属中相互交织的有序状态。

Disentangling the intertwined orders in a magnetic kagome metal.

作者信息

Oh Ji Seop, Biswas Ananya, Klemm Mason L, Tan Hengxin, Xie Yaofeng, Gao Bin, Hashimoto Makoto, Lu Donghui, Yan Binghai, Dai Pengcheng, Birgeneau Robert J, Yi Ming

机构信息

Department of Physics, University of California, Berkeley, CA 94720, USA.

Department of Physics and Astronomy and Smalley-Curl Institute, Rice University, Houston, TX 77005, USA.

出版信息

Sci Adv. 2025 Jul 4;11(27):eadt2195. doi: 10.1126/sciadv.adt2195. Epub 2025 Jul 2.

Abstract

Intertwined orders appear when multiple orders are strongly interacting, and kagome metals have emerged as new platforms to explore exotic phases. FeGe has been found to develop a charge density wave (CDW) order within magnetic phase, suggesting an intricate interplay of the lattice, charge, and spin degrees of freedom. Recently, postgrowth annealing has been proposed to tune the CDW order from long-range to complete suppression, offering a tuning knob for the CDW order. Here, by comparing the electronic structures of FeGe subjected to different annealing conditions and distinct CDW properties, we report spectral evolution associated with the lattice and spin degrees of freedom. We find band evolution linked to a spin density wave (SDW) order present in both samples with and without CDW order, and another evolution connected to the lattice distortions that onset with the long-range CDW order and revert with the SDW order. Our results reveal a rare competitive cooperation of the lattice, spin, and charge in FeGe.

摘要

当多个序强烈相互作用时会出现交织序,而 Kagome 金属已成为探索奇异相的新平台。人们发现 FeGe 在磁相内会形成电荷密度波(CDW)序,这表明晶格、电荷和自旋自由度之间存在复杂的相互作用。最近,有人提出生长后退火可将 CDW 序从长程调至完全抑制,为 CDW 序提供了一个调节旋钮。在此,通过比较处于不同退火条件且具有不同 CDW 特性的 FeGe 的电子结构,我们报告了与晶格和自旋自由度相关的光谱演化。我们发现,在有和没有 CDW 序的样品中都存在与自旋密度波(SDW)序相关的能带演化,以及另一种与晶格畸变相关的演化,这种晶格畸变随着长程 CDW 序的出现而开始,并随着 SDW 序的恢复而恢复。我们的结果揭示了 FeGe 中晶格、自旋和电荷之间罕见的竞争合作关系。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d2a0/12219475/34e3c6fa7972/sciadv.adt2195-f1.jpg

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