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采用碳捕获和碳升级循环工艺的混凝土生产生命周期评估

Life-cycle assessment of concrete production with carbon capture and carbon upcycling process.

作者信息

Chen Tianyu, Nelson Jacob P, Gupta Vijay, Mobley Paul D

机构信息

RTI International, 3040 E. Cornwallis Rd, Research Triangle Park, NC, 27713, USA.

RTI International, 3040 E. Cornwallis Rd, Research Triangle Park, NC, 27713, USA.

出版信息

J Environ Manage. 2025 Sep;391:126303. doi: 10.1016/j.jenvman.2025.126303. Epub 2025 Jul 2.

Abstract

The main CO utilization methods for concrete production, aimed at reducing its carbon footprint, include several promising approaches. These methods include the carbonation of concrete, where CO reacts with calcium hydroxide to form calcium carbonate; CO-activated concrete, achieved by infusion of CO into concrete during the mixing or curing process; and carbonation of recycled concrete, which uses industrial byproducts like slag and fly ash to sequester CO. Another method is the use of biochar in concrete, where CO is sequestered from organic waste to enhance material properties. More recently, a new method has emerged where CO is used to transform industrial byproducts into enhanced supplementary cementitious materials (SCMs) that are then used to either produce blended cements or used directly in concrete. These techniques not only lower carbon emissions but also have the potential to enhance the strength and durability of concrete, making it even more desirable for construction applications. A significant reduction in the CO intensity of concrete production can be achieved by using post-combustion CO capture processes to capture the CO emissions from the cement production process. A life-cycle assessment (LCA) methodology is crucial to assess and mitigate the environmental impact of concrete. Various decision makers and manufacturers are keenly interested in using an LCA approach to understand and minimize the ecological footprint of concrete.

摘要

旨在减少混凝土碳足迹的主要CO利用方法包括几种有前景的途径。这些方法包括混凝土的碳酸化,即CO与氢氧化钙反应形成碳酸钙;CO活化混凝土,通过在搅拌或养护过程中将CO注入混凝土中实现;以及再生混凝土的碳酸化,其利用矿渣和粉煤灰等工业副产品来封存CO。另一种方法是在混凝土中使用生物炭,从有机废物中封存CO以增强材料性能。最近,出现了一种新方法,即利用CO将工业副产品转化为增强型辅助胶凝材料(SCMs),然后用于生产混合水泥或直接用于混凝土中。这些技术不仅降低了碳排放,还有潜力提高混凝土的强度和耐久性,使其在建筑应用中更具吸引力。通过使用燃烧后CO捕集工艺来捕集水泥生产过程中的CO排放,可以显著降低混凝土生产的CO强度。生命周期评估(LCA)方法对于评估和减轻混凝土的环境影响至关重要。各种决策者和制造商对使用LCA方法来理解和最小化混凝土的生态足迹非常感兴趣。

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