Suppr超能文献

基于静电纺丝制备的AgO和PtO共修饰LaFeO纳米纤维的高灵敏度甲醛气体传感器

A Highly Sensitive Formaldehyde Gas Sensor Based on AgO and PtO Co-Decorated LaFeO Nanofibers Prepared by Electrospinning.

作者信息

Wang Xin, Song Fei, Fu Huai'an, Yu Shanshan, Zhang Kai, Tang Zhipeng, Meng Qingkuan, Jing Qiang, Liu Bo

机构信息

Laboratory of Functional Molecules and Materials, School of Physics and Optoelectronic Engineering, Shandong University of Technology, 266 Xincun Xi Road, Zibo 255000, China.

School of Mathematics and Physics, Xi'an Jiaotong-Liverpool University, Suzhou 215123, China.

出版信息

Sensors (Basel). 2025 Jun 20;25(13):3848. doi: 10.3390/s25133848.

Abstract

The widespread use of formaldehyde in both industrial and household products has raised significant health concerns, emphasizing the need for highly sensitive sensors to monitor formaldehyde concentrations in the environment in real time. In this study, we report the fabrication of a highly sensitive formaldehyde gas sensor based on AgO and PtO co-decorated LaFeO nanofibers, prepared by electrospinning, with an ultra-low detection limit of 10 ppb. Operating at an optimal temperature of 210 °C, the sensor exhibits high sensitivity, with a response value of 283 to 100 ppm formaldehyde-nearly double the response of the Ag-only decorated LaFeO sensor. Additionally, the sensor demonstrated good selectivity, repeatability, and long-term stability over 80 days. The enhanced sensitivity is attributed to the strong adsorption ability of Ag towards both oxygen and formaldehyde, Ag's catalytic oxidation of formaldehyde, PtO's catalytic action on oxygen, and the spillover effect of PtO on oxygen. This sensor holds significant potential for environmental monitoring due to its ultrahigh sensitivity and ease of fabrication.

摘要

甲醛在工业和家用产品中的广泛使用引发了重大的健康担忧,这凸显了对高灵敏度传感器的需求,以便实时监测环境中的甲醛浓度。在本研究中,我们报告了一种基于AgO和PtO共修饰的LaFeO纳米纤维制备的高灵敏度甲醛气体传感器,该传感器通过静电纺丝制备,具有10 ppb的超低检测限。在210 °C的最佳温度下运行时,该传感器表现出高灵敏度,对100 ppm甲醛的响应值为283,几乎是仅用Ag修饰的LaFeO传感器响应值的两倍。此外,该传感器在80天内表现出良好的选择性、重复性和长期稳定性。灵敏度的提高归因于Ag对氧气和甲醛的强吸附能力、Ag对甲醛的催化氧化、PtO对氧气的催化作用以及PtO对氧气的溢流效应。由于其超高灵敏度和易于制备,该传感器在环境监测方面具有巨大潜力。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9526/12251707/d693399cb4e2/sensors-25-03848-g001.jpg

文献AI研究员

20分钟写一篇综述,助力文献阅读效率提升50倍。

立即体验

用中文搜PubMed

大模型驱动的PubMed中文搜索引擎

马上搜索

文档翻译

学术文献翻译模型,支持多种主流文档格式。

立即体验