Zhao Weiyao, Xing Kaijian, Zhao Yufei, Chen Lei, Hong Min, Yin Yuefeng, Liu Yang, Le Dang Khoa, Gayles Jacob, Tang Fang, Fang Yong, Yan Binghai, Karel Julie
Department of Materials Science & Engineering, & ARC Centre of Excellence in Future Low-Energy Electronics Technologies, Monash University, Clayton, VIC, Australia.
School of Physics & Astronomy, Monash University, Clayton, VIC, Australia.
Nat Commun. 2025 Jul 24;16(1):6837. doi: 10.1038/s41467-025-62096-z.
Quantum geometry, including Berry curvature and the quantum metric, of the electronic Bloch bands has been studied via nonlinear responses in topological materials. Naturally, these material systems with intrinsic strong nonlinear responses also form the key component in nonlinear electronic devices. However, the previous reported quantum geometry effects are mainly observed at cryogenic temperatures, hindering their application in practical devices. Here we report a tuneable strong room-temperature second-harmonic transport response in a quantum magnet, TbMnSn, which is governed by the quantum metric and can be tuned with applied magnetic fields. We show that around room temperature, which is close to the spontaneous spin-reorientation transition, the magnetic configurations, and therefore the related symmetry breaking phases, are easily controlled via magnetic fields. Our results also show that manipulation of the symmetries of the magnetic structure presents an effective route to tuneable quantum-geometry-based devices.
通过拓扑材料中的非线性响应,对电子布洛赫能带的量子几何(包括贝里曲率和量子度量)进行了研究。自然而然地,这些具有固有强非线性响应的材料系统也构成了非线性电子器件的关键组成部分。然而,先前报道的量子几何效应主要是在低温下观察到的,这阻碍了它们在实际器件中的应用。在此,我们报告了一种量子磁体TbMnSn中可调节的强室温二次谐波输运响应,该响应由量子度量控制,并且可以通过施加磁场进行调节。我们表明,在接近室温且接近自发自旋重取向转变的温度下,磁构型以及因此相关的对称破缺相很容易通过磁场进行控制。我们的结果还表明,操纵磁结构的对称性为基于量子几何的可调节器件提供了一条有效途径。