He Jiahui, Han Xiaojing, Jiang Yunlu, Ren Aoyu, Yang Zhengyang, Zhang Zhenyu, Wang Mei, Yang Bin, Yin Minzhen, Peng Huasheng, Huang Luqi
School of Pharmacy, Anhui University of Chinese Medicine, Hefei 230012, China.
State Key Laboratory for Quality Ensurance and Sustainable Use of Dao-di Herbs, National Resource Center for Chinese Materia Medica, China Academy of Chinese Medical Sciences, Beijing 100700, China.
J Agric Food Chem. 2025 Aug 20;73(33):20745-20755. doi: 10.1021/acs.jafc.5c05277. Epub 2025 Aug 7.
Tracing agricultural products' origin via Sr/Sr is critical for food quality. This study identifies optimal proxy samples for baseline maps by analyzing Sr isotopes in three vegetation life-forms (perennial herbs, shrubs, trees) and their soils under diverse parent materials. The results indicate significant differences in Sr-isotopic composition between roots and soils, likely due to the heterogeneous geological origin of eolian soils. Trees and shrubs grown on residual parent materials exhibit homogeneous isotopic signatures across organs, with Sr/Sr ratios strongly correlated ( > 0.85) with mixed surface vegetation samples. Thus, this study demonstrates that Sr/Sr isoscapes constructed from multispecies vegetation sampling overcome methodological constraints arising from seasonal variations in agricultural traceability. These findings establish a theoretical foundation for a cross-plant-type origin-tracing framework capable of harmonizing divergent crop data sets and have implications for refining the methodology of botanical Sr sourcing.
通过锶同位素比值(Sr/Sr)追踪农产品来源对食品质量至关重要。本研究通过分析三种植被生命形式(多年生草本植物、灌木、树木)及其在不同母质下的土壤中的锶同位素,确定了用于基线地图的最佳替代样本。结果表明,根与土壤之间的锶同位素组成存在显著差异,这可能是由于风积土的地质来源不均一所致。生长在残留母质上的树木和灌木在各器官间呈现出均匀的同位素特征,其Sr/Sr比值与混合地表植被样本高度相关(>0.85)。因此,本研究表明,由多物种植被采样构建的Sr/Sr等时线图克服了农业溯源中季节性变化带来的方法学限制。这些发现为能够协调不同作物数据集的跨植物类型溯源框架奠定了理论基础,并对完善植物性锶源追踪方法具有启示意义。