Deng Zixuan, Priimagi Arri, Li Kai, Zeng Hao
Faculty of Engineering and Natural Sciences, Tampere University, Tampere, Finland.
School of Civil Engineering, Anhui Jianzhu University, Hefei, China.
Commun Mater. 2025;6(1):173. doi: 10.1038/s43246-025-00903-2. Epub 2025 Aug 5.
Light-responsive materials with intrinsic negative feedback enable self-oscillation in non-equilibrium states. Conventional systems rely on self-shadowing in bending modes but fail when shadowing is constrained. Here, we demonstrate that external mechanical forces can bypass this limitation, enabling sustained oscillations without complete shadowing. Using a vertically suspended light-responsive liquid crystal network (LCN) strip under constant irradiation, a transition from static deformation to continuous oscillation arises when a critical load is applied. This system reveals two key phenomena: (1) oscillation amplitude scales with light intensity, reaching an angular displacement of 300°-significantly surpassing bending-mode oscillators; and (2) oscillation frequency decreases with increasing load, reflecting intrinsic mechanical sensitivity. This force-assisted self-oscillation principle generalizes across diverse deformation modes, including bending, twisting, contraction, and off-axis LCN strips. By mimicking biological mechanosensation based on dissipative mechanism, our findings provide a simplified design for non-equilibrium matter capable of dynamic adaptation to mechanical loads.
具有内在负反馈的光响应材料能够在非平衡状态下实现自振荡。传统系统依靠弯曲模式下的自遮挡,但当遮挡受到限制时就会失效。在此,我们证明外部机械力可以绕过这一限制,在没有完全遮挡的情况下实现持续振荡。在恒定光照下使用垂直悬挂的光响应液晶网络(LCN)条带,当施加临界载荷时,会出现从静态变形到连续振荡的转变。该系统揭示了两个关键现象:(1)振荡幅度与光强度成比例,达到300°的角位移——显著超过弯曲模式振荡器;(2)振荡频率随载荷增加而降低,反映出内在的机械敏感性。这种力辅助自振荡原理适用于多种变形模式,包括弯曲、扭转、收缩和离轴LCN条带。通过模仿基于耗散机制的生物机械传感,我们的发现为能够动态适应机械载荷的非平衡物质提供了一种简化设计。