Murata Masayuki, Ando Fuyuki, Hirai Takamasa, Adachi Hiroto, Uchida Ken-Ichi
Research Institute for Energy Conservation, National Institute of Advanced Industrial Science and Technology, Tsukuba, Japan.
Research Center for Magnetic and Spintronic Materials, National Institute for Materials Science, Tsukuba, Japan.
Sci Technol Adv Mater. 2025 Jul 29;26(1):2535955. doi: 10.1080/14686996.2025.2535955. eCollection 2025.
The transverse thermoelectric generation and cooling performances in a thermopile module composed of recently developed SmCo/BiSbTe artificially tilted multilayers are evaluated quantitatively. When a large temperature difference of 405°C is applied to the SmCo/BiSbTe-based module, the open-circuit voltage and output power reach 0.51 V and 0.80 W, respectively. The corresponding maximum power density is 0.16 W/cm, even if the power is normalized by the device area including areas that do not contribute to the power generation, such as epoxy resin, electrodes, and insulating layers. The maximum energy conversion efficiency for our module in this condition is experimentally determined to be 0.92%. Under the cooling operation, the same module exhibits the maximum temperature difference of 9.0°C and heat flow at the cold side of 1.6 W. Although these values are lower than the ideal thermoelectric performance expected from the material parameters due to the imperfections associated with modularization, the systematic investigations reported here clarify a potential of the SmCo/BiSbTe artificially tilted multilayers as thermoelectric generators and cooling devices.
对由最近开发的SmCo/BiSbTe人工倾斜多层膜组成的热电堆模块中的横向热电发电和冷却性能进行了定量评估。当对基于SmCo/BiSbTe的模块施加405°C的大温差时,开路电压和输出功率分别达到0.51 V和0.80 W。即使通过包括环氧树脂、电极和绝缘层等不参与发电区域的器件面积对功率进行归一化,相应的最大功率密度仍为0.16 W/cm。在此条件下,我们模块的最大能量转换效率经实验测定为0.92%。在冷却运行下,同一模块的最大温差为9.0°C,冷侧的热流为1.6 W。尽管由于与模块化相关的缺陷,这些值低于根据材料参数预期的理想热电性能,但本文报道的系统研究阐明了SmCo/BiSbTe人工倾斜多层膜作为热电发电机和冷却装置的潜力。