Löscher Robin, Schroeder Malte C, Vogel Tim, Omar Alan, Hasso Adam, Hoberg Claudius, Havenith Martina, Saraceno Clara J
Opt Express. 2025 Mar 10;33(5):9213-9223. doi: 10.1364/OE.546773.
Ultrafast THz transients with large spectral bandwidths are commonly generated in the two-color air-plasma scheme, typically driven by high-pulse-energy laser sources, operating at low repetition rates up to a few kHz. The low repetition rate of these sources is a strong limiting factor to reaching high dynamic ranges in measurements involving long integration times or multi-dimensional scans. The advent of high-power Yb-based laser sources in combination with nonlinear temporal compression schemes opens the door to air-plasma THz sources at significantly higher repetition rates up to hundreds of kHz and beyond. In this study, we investigate for the first time repetition rate scaling in the two-color filament plasma scheme at repetition rates ranging from 1 kHz up to 100 kHz. We study the influence of repetition rate on THz yield and observe a correlation between the decrease of the optical-to-THz conversion efficiency and the gas density depletion in the filamentation region that we measure using interferometry. The experimentally observed optical-to-THz conversion efficiencies are in approximate agreement with a simple one-dimensional photocurrent model we developed. These findings set the foundation for future repetition rate scaling experiments towards the MHz region, using the broadband and affordable two-color air-plasma scheme. At 100 kHz, we generate THz radiation with a maximum average power of 2.8 mW and peak electric fields reaching 165 kV/cm. Using electro-optic sampling, we detect frequencies up to 23 THz, showing the broadband nature of the source. This source is a promising alternative both for future linear and nonlinear ultra-broadband spectroscopic investigations at greatly accelerated measurement times.
具有大光谱带宽的超快太赫兹瞬态通常在双色空气等离子体方案中产生,通常由高脉冲能量激光源驱动,工作在高达几千赫兹的低重复率下。这些源的低重复率是在涉及长积分时间或多维扫描的测量中达到高动态范围的一个强大限制因素。高功率镱基激光源与非线性时间压缩方案的出现,为重复率高达数百千赫兹及以上的空气等离子体太赫兹源打开了大门。在本研究中,我们首次研究了双色丝状等离子体方案中从1千赫兹到100千赫兹重复率范围内的重复率缩放。我们研究了重复率对太赫兹产率的影响,并观察到光到太赫兹转换效率的降低与我们使用干涉测量法测量的丝状区域中的气体密度耗尽之间的相关性。实验观察到的光到太赫兹转换效率与我们开发的一个简单的一维光电流模型大致相符。这些发现为未来使用宽带且经济实惠的双色空气等离子体方案向兆赫兹区域进行重复率缩放实验奠定了基础。在100千赫兹时,我们产生了最大平均功率为2.8毫瓦且峰值电场达到165千伏/厘米的太赫兹辐射。使用电光采样,我们检测到高达23太赫兹的频率,显示了该源的宽带特性。该源对于未来在大大加快测量时间的情况下进行线性和非线性超宽带光谱研究都是一个有前途的替代方案。