Zheng Chao, Gao Shuilian, Wang Xiaxia, Yang Zhenbiao, Zhou Junling, Liu Ying
Haixia Institute of Science and Technology, Fujian Agriculture and Forestry University, Fuzhou 350007, China.
Anxi College of Tea Science, Fujian Agriculture and Forestry University, Fuzhou 350007, China.
Plants (Basel). 2025 Aug 1;14(15):2378. doi: 10.3390/plants14152378.
The impact of seasonality on the aroma quality of tea has been documented in various tea types, but not specifically in oolong tea. This study is the first to explore the complex relationships between seasonality, volatile compounds, and aroma quality in oolong tea. Using Headspace Solid-Phase Microextraction Gas Chromatography-Mass Spectrometry (HS-SPME-GC-MS)-based untargeted metabolomics, we analyzed 266 samples of Tieguanyin oolong tea. The data identified linalool, linalool oxides (trans-linalool oxide (furanoid) and trans-linalool oxide (pyranoid)), and their metabolites (diendiol I; hotrienol) as key seasonal discriminants. Four out of the top ten key differential compounds for distinguishing aroma scores were metabolites from fatty acid degradation, namely trans-3-hexenyl butyrate, trans-2-hexenyl hexanoate, hexyl hexanoate, and hexyl 2-methyl butyrate. Approximately one-fifth of the seasonal discriminant volatile compounds were significant in influencing aroma quality. Overall, the impact of seasonality on the aroma quality of finished Tieguanyin oolong tea is marginal. These findings enhance our understanding of the interplay between seasonal variations, volatile composition, and aroma quality in oolong tea.
季节性对各类茶叶香气品质的影响已有文献记载,但在乌龙茶方面尚无具体研究。本研究首次探讨了季节性、挥发性化合物与乌龙茶香气品质之间的复杂关系。我们采用基于顶空固相微萃取气相色谱 - 质谱联用(HS - SPME - GC - MS)的非靶向代谢组学方法,分析了266份铁观音乌龙茶样品。数据鉴定出芳樟醇、芳樟醇氧化物(反式芳樟醇氧化物(呋喃型)和顺式芳樟醇氧化物(吡喃型))及其代谢产物(二氢二醇I;热rienol)为关键的季节性判别指标。用于区分香气得分的前十大关键差异化合物中有四种是脂肪酸降解的代谢产物,即反式 - 3 - 己烯基丁酸酯、反式 - 2 - 己烯基己酸酯、己基己酸酯和己基2 - 甲基丁酸酯。约五分之一的季节性判别挥发性化合物对香气品质有显著影响。总体而言,季节性对成品铁观音乌龙茶香气品质的影响较小。这些发现增进了我们对乌龙茶季节性变化、挥发性成分和香气品质之间相互作用的理解。