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直接测量羽流速度以表征点源排放。

Direct measurement of plume velocity to characterize point source emissions.

作者信息

Eastwood Michael L, Thompson David R, Green Robert O, Fahlen Jay E, Adams Taylor J, Brandt Adam R, Brodrick Philip G, Chlus Adam, Kort Eric A, Reuland Frances, Thorpe Andrew K

机构信息

Jet Propulsion Laboratory, California Institute of Technology, Pasadena, CA 91109.

Climate and Space Sciences and Engineering, University of Michigan, Ann Arbor, MI 48109.

出版信息

Proc Natl Acad Sci U S A. 2025 Sep 9;122(36):e2507350122. doi: 10.1073/pnas.2507350122. Epub 2025 Sep 2.

DOI:10.1073/pnas.2507350122
PMID:40892911
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12435211/
Abstract

An explosion of recent research uses remote imaging spectroscopy from aircraft and spacecraft to detect and quantify methane point source emissions. These instruments first map the methane enhancement field and then combine this information with the effective wind speed to estimate the source emission rate. This wind speed is typically the largest uncertainty in derived emission rates. It is often, by necessity, inferred from coarse-resolution meteorological reanalysis products which do not match the spatial or temporal extent of wind experienced by the gas plume. Here, we circumvent this problem by simultaneously measuring plume velocity using the same spectrometer that maps the methane plume. Our approach acquires multiple consecutive views of the same point source, with visual tracking of the plume's features to estimate its ground velocity. This resolves the representational mismatch between reanalysis and effective wind speeds. It provides data with exact spatiotemporal coincidence to the plume being measured. The approach facilitates dramatic improvement in the precision of remote methane point source quantification.

摘要

最近大量的研究利用来自飞机和航天器的遥感成像光谱技术来检测和量化甲烷点源排放。这些仪器首先绘制甲烷增强场图,然后将此信息与有效风速相结合,以估算源排放率。这种风速通常是推导排放率中最大的不确定因素。由于需要,它通常是从粗分辨率气象再分析产品中推断出来的,而这些产品与气团所经历的风的空间或时间范围不匹配。在此,我们通过使用绘制甲烷羽流的同一光谱仪同时测量羽流速度来规避这个问题。我们的方法获取同一点源的多个连续视图,通过对羽流特征的视觉跟踪来估算其地面速度。这解决了再分析风速与有效风速之间的代表性不匹配问题。它提供了与被测羽流在时空上精确重合的数据。该方法有助于显著提高远程甲烷点源量化的精度。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a895/12435211/762e314e965f/pnas.2507350122fig02.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a895/12435211/a07f8690ed37/pnas.2507350122fig01.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a895/12435211/762e314e965f/pnas.2507350122fig02.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a895/12435211/a07f8690ed37/pnas.2507350122fig01.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a895/12435211/762e314e965f/pnas.2507350122fig02.jpg

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本文引用的文献

1
Technological Maturity of Aircraft-Based Methane Sensing for Greenhouse Gas Mitigation.飞机甲烷探测技术在温室气体减排中的成熟度。
Environ Sci Technol. 2024 Jun 4;58(22):9591-9600. doi: 10.1021/acs.est.4c02439. Epub 2024 May 17.
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Geostationary satellite observations of extreme and transient methane emissions from oil and gas infrastructure.地球静止卫星对石油和天然气基础设施的极端和瞬时甲烷排放的观测。
Proc Natl Acad Sci U S A. 2023 Dec 26;120(52):e2310797120. doi: 10.1073/pnas.2310797120. Epub 2023 Dec 19.
3
Attribution of individual methane and carbon dioxide emission sources using EMIT observations from space.
利用来自太空的EMIT观测数据对甲烷和二氧化碳单个排放源进行归因。
Sci Adv. 2023 Nov 15;9(46):eadh2391. doi: 10.1126/sciadv.adh2391. Epub 2023 Nov 17.
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Are Optical Gas Imaging Technologies Effective For Methane Leak Detection?光学气体成像技术在甲烷泄漏检测方面是否有效?
Environ Sci Technol. 2017 Jan 3;51(1):718-724. doi: 10.1021/acs.est.6b03906. Epub 2016 Dec 12.
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Airborne methane remote measurements reveal heavy-tail flux distribution in Four Corners region.机载甲烷遥感测量揭示四角地区的重尾通量分布。
Proc Natl Acad Sci U S A. 2016 Aug 30;113(35):9734-9. doi: 10.1073/pnas.1605617113. Epub 2016 Aug 15.