Travin Dmitrii Y, Basu Ritwika S, Paranjpe Madhura N, Klepacki Dorota, Zhurakovskaya Anna I, Vázquez-Laslop Nora, Mankin Alexander S, Polikanov Yury S, Gagnon Matthieu G
Department of Pharmaceutical Sciences, University of Illinois at Chicago, Chicago, IL 60607, USA.
Center for Biomolecular Sciences, University of Illinois at Chicago, Chicago, IL 60607, USA.
bioRxiv. 2025 Aug 20:2025.08.17.670399. doi: 10.1101/2025.08.17.670399.
The development of antibiotics with novel mechanisms of action is essential to address the growing threat of antimicrobial resistance. Protein synthesis-inhibiting antibiotic bottromycin (BOT), a ribosomally synthesized and posttranslationally modified peptide (RiPP), has long been known for its potent activity against Gram-positive bacteria but was largely neglected due in part to the lack of understanding of its mechanism of action. Here we uncover the unprecedented mode translation inhibition strategy employed by BOT. Using biochemical, microbiological, genetic, and structural approaches, we show that BOT acts by selectively trapping elongation factor-Tu (EF-Tu) in complex with glycyl-tRNA on the ribosome. BOT binds at the interface between EF-Tu and the CCA-end of Gly-tRNA, stabilizing the EF-Tu/Gly-tRNA complex in a pre-accommodated A/T-state on the ribosome, and specifically arresting translation at glycine codons. This mode of action is mechanistically distinct from that of other EF-Tu-targeting antibiotics, which act in a tRNA-agnostic fashion. Point mutations in EF-Tu confer high-level resistance to BOT, confirming EF-Tu as the direct and essential target of the drug. Our findings establish BOT as a founding member of a new class of antibiotics that stall the ribosome at defined mRNA sites by trapping a specific elongation factor-tRNA complex.
开发具有新型作用机制的抗生素对于应对日益严重的抗菌药物耐药性威胁至关重要。蛋白质合成抑制抗生素波卓霉素(BOT)是一种核糖体合成且经过翻译后修饰的肽(RiPP),长期以来因其对革兰氏阳性菌具有强大活性而闻名,但部分由于对其作用机制缺乏了解而在很大程度上被忽视。在此,我们揭示了BOT所采用的前所未有的翻译抑制策略。通过生物化学、微生物学、遗传学和结构学方法,我们表明BOT的作用方式是在核糖体上选择性地捕获与甘氨酰 - tRNA结合的延伸因子 - Tu(EF - Tu)。BOT结合在EF - Tu与甘氨酰 - tRNA的CCA末端之间的界面处,将EF - Tu/甘氨酰 - tRNA复合物稳定在核糖体上预先容纳的A/T状态,并特异性地在甘氨酸密码子处阻止翻译。这种作用方式在机制上与其他靶向EF - Tu的抗生素不同,后者以不依赖tRNA的方式起作用。EF - Tu中的点突变赋予对BOT的高水平抗性,证实EF - Tu是该药物的直接且必需的靶点。我们的研究结果确立了BOT作为一类新型抗生素的创始成员,这类抗生素通过捕获特定的延伸因子 - tRNA复合物在特定的mRNA位点使核糖体停滞。