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硫酸钙:镝聚四氟乙烯热释光剂量计的热历史和可重复使用性

Thermal history and reusability of CaSO4: Dy Teflon TLD discs.

作者信息

Lakshmanan A R, Popli K L, Bhatt R C

出版信息

Phys Med Biol. 1979 Sep;24(5):999-1008. doi: 10.1088/0031-9155/24/5/012.

Abstract

The TL sensitivity of CaCO4 : Dy Teflon TLD discs was found not to change after isothermal annealing for 1 h in the temperature range 220--400 degrees C. The reusability of these TLD discs after two separate annealing treatments (240 degrees C and 400 degrees C, each 1 h) were studied for 20 cycles of use. The former annealing treatment resulted in a 12% loss in TL sensitivity after 20 cycles, mainly due to the increase in optical density of these discs. A decrease in the maximum temperature from 300 to 250 degrees C while clamped for read-out in the TLD reader has prevented any change in the optical density of these discs, and their TL sensitivity did not show any change after 20 cycles. The darkening of PTFE-based TL dosemeters was attributed to the reorientation of molecules in PTFE when the temperature during readout exceeds 250 degrees C; isothermal annealing at 400 degrees C restored their original colour. Their TL sensitivity decreased gradually with the number of cycles (over 15% in 20 cycles) after the 400 degrees C anneal, mainly because of the loss in TL sensitivity of the CaSO4 : Dy phosphor itself. This study has demonstrated that under controlled conditions, the Teflon TL dosemeters can be reused a number of times without any change in TL sensitivity.

摘要

发现CaCO4 : Dy聚四氟乙烯热释光剂量计圆盘在220 - 400摄氏度温度范围内等温退火1小时后,其热释光(TL)灵敏度没有变化。研究了这些热释光剂量计圆盘在两次单独的退火处理(240摄氏度和400摄氏度,每次1小时)后20次使用循环的可重复使用性。前一种退火处理导致在20次循环后热释光灵敏度损失12%,主要是由于这些圆盘的光密度增加。在热释光读数器中夹紧读出时,将最高温度从300摄氏度降至250摄氏度,防止了这些圆盘光密度的任何变化,并且它们的热释光灵敏度在20次循环后没有显示出任何变化。基于聚四氟乙烯的热释光剂量计的变黑归因于读出期间温度超过250摄氏度时聚四氟乙烯中分子的重新取向;在400摄氏度等温退火恢复了它们原来的颜色。在400摄氏度退火后,它们的热释光灵敏度随着循环次数逐渐降低(20次循环中超过15%),主要是因为CaSO4 : Dy磷光体本身热释光灵敏度的损失。这项研究表明,在受控条件下,聚四氟乙烯热释光剂量计可以多次重复使用而热释光灵敏度没有任何变化。

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