Spicer C W
Sci Total Environ. 1982 Jun;24(2):183-92. doi: 10.1016/0048-9697(82)90110-3.
This paper describes the distribution of oxidized nitrogen compounds in urban air. The studies reported here have focused on NO, NO2, PAN and NO-3. These species have been monitored for periods of several weeks at a nmber of locations throughout the U.S.A. Oxidized nitrogen distribution is discussed in terms of the daily patterns of nitrogen pollutant concentrations, the fractional conversion of NOx to products and the diurnal profile of the conversion fraction, and lastly, the contribution of the individual compounds to the overall oxidized nitrogen burden. Site to site variations in the distribution are explained by photochemical conversion, distance between the site and the source region, and the proximity of local NOx emission sources.
本文描述了城市空气中氧化态氮化合物的分布情况。此处报道的研究聚焦于一氧化氮(NO)、二氧化氮(NO₂)、过氧乙酰硝酸酯(PAN)和硝酸根(NO₃⁻)。在美国多个地点对这些物种进行了为期数周的监测。从氮污染物浓度的每日变化模式、氮氧化物(NOₓ)向产物的转化分数以及转化分数的日变化曲线,最后是各个化合物对总氧化态氮负荷的贡献等方面讨论了氧化态氮的分布。分布的站点间差异通过光化学转化、站点与源区之间的距离以及当地氮氧化物排放源的 proximity 来解释。 (注:原文中“proximity”直译为“接近度”,此处结合语境推测是指当地氮氧化物排放源的距离远近等情况,但原词有误,正确的应该是“proximity”,意为“接近;临近” )