Rees D C, Lewis M, Honzatko R B, Lipscomb W N, Hardman K D
Proc Natl Acad Sci U S A. 1981 Jun;78(6):3408-12. doi: 10.1073/pnas.78.6.3408.
The structure of the metalloenzyme carboxypeptidase A (peptidyl-L-amino-acid hydrolase, EC 3.4.17.1) has been refined at 1.75 A by a restrained least-squares procedure to a conventional crystallographic R factor of 0.162. Significant results of the refined structure relative to the catalytic mechanism are described. In the native enzyme, the zinc coordination number is five (two imidazole N delta 1 nitrogens, the two carboxylate oxygens of glutamate-72, and a water molecule). In the complex (at 2.0-A resolution) of carboxypeptidase A with the dipeptide glycyl-L-tyrosine, however, the water ligand is replaced by both the carbonyl oxygen and the amino nitrogen of the dipeptide. The amino nitrogen also statistically occupies a second position near glutamate-270. Consequently, the coordination number of zinc may vary from five to six in carboxypeptidase A-substrate complexes. Implications of these results for the catalytic mechanism of carboxypeptidase A are discussed. In addition, three cis peptide bonds, none of which involves proline as the amino nitrogen donor, have been located fairly near the active site.
金属酶羧肽酶A(肽基-L-氨基酸水解酶,EC 3.4.17.1)的结构已通过约束最小二乘法在1.75 Å分辨率下进行了精修,传统晶体学R因子为0.162。描述了相对于催化机制的精修结构的重要结果。在天然酶中,锌的配位数为五(两个咪唑Nδ1氮原子、谷氨酸-72的两个羧基氧原子和一个水分子)。然而,在羧肽酶A与二肽甘氨酰-L-酪氨酸的复合物(分辨率为2.0 Å)中,水配体被二肽的羰基氧原子和氨基氮原子取代。氨基氮原子在统计学上也占据了靠近谷氨酸-270的第二个位置。因此,在羧肽酶A-底物复合物中,锌的配位数可能从五变为六。讨论了这些结果对羧肽酶A催化机制的影响。此外,在活性位点附近相当近的位置发现了三个顺式肽键,其中没有一个涉及脯氨酸作为氨基氮供体。