Bellingham R M, Gibbs A H, de Matteis F, Lian L Y, Roberts G C
Biological NMR Centre, University of Leicester, UK.
Biochem J. 1995 Apr 15;307 ( Pt 2)(Pt 2):505-12. doi: 10.1042/bj3070505.
Feeding mice with griseofulvin, a widely used anti-fungal agent which induces protoporphyria as a side-effect, leads to the formation in the liver of two green pigments which have been shown to be porphyrin adducts. In this work, the major porphyrin adduct isolated from the livers of griseofulvin-fed mice has been characterized structurally using one- and two-dimensional NMR spectroscopy. The adduct was shown to be an N-alkylated protoporphyrin IX in which the whole of griseofulvin (less a hydrogen atom) is attached to a pyrrole ring nitrogen of the porphyrin. It was shown that the drug-to-porphyrin linkage is an an -O-CH2-Npyrrole = linkage, to either the 4- or 6-position of ring a of griseofulvin. In an attempt to identify which pyrrole nitrogen is involved in this linkage, the 1H spectra of the free base and zinc complex of the adduct were compared with the corresponding spectra of the four regioisomers of N-methylprotoporphyrin. These comparisons indicated that the adduct isolated from the livers of griseofulvin-fed mice is either the NC or the ND regioisomer, although a clear distinction between these two could not be made on the available evidence. The mechanism of formation of the adduct and its relation to griseofulvin-induced protoporphyria are discussed.
用灰黄霉素喂养小鼠,灰黄霉素是一种广泛使用的抗真菌剂,会作为副作用诱发原卟啉症,这会导致在肝脏中形成两种绿色色素,已证明它们是卟啉加合物。在这项工作中,从用灰黄霉素喂养的小鼠肝脏中分离出的主要卟啉加合物已通过一维和二维核磁共振光谱进行了结构表征。该加合物被证明是一种N-烷基化原卟啉IX,其中整个灰黄霉素(少一个氢原子)连接到卟啉的一个吡咯环氮上。结果表明,药物与卟啉的连接是一种-O-CH2-Npyrrole =连接,连接到灰黄霉素a环的4位或6位。为了确定哪个吡咯氮参与了这种连接,将加合物的游离碱和锌配合物的1H光谱与N-甲基原卟啉的四种区域异构体的相应光谱进行了比较。这些比较表明,从用灰黄霉素喂养的小鼠肝脏中分离出的加合物要么是NC区域异构体,要么是ND区域异构体,尽管根据现有证据无法在这两者之间做出明确区分。讨论了加合物的形成机制及其与灰黄霉素诱导的原卟啉症的关系。