Sun H
Department of Geology, Florida State University, Tallahassee 32306.
Health Phys. 1995 Apr;68(4):553-60. doi: 10.1097/00004032-199504000-00013.
Prediction of radon release from building materials is a general problem. Since it is impractical to follow each recoil radon path and measure the surface area of porous texture by experimental methods, a powerful computer simulation approach is conducted in this paper. The Monte Carlo simulation program TRIM, based on the momentum and energy conservation of the ion transport in matter, is modified to simulate the recoil path in a 3-D frame. A follow-up Monte Carlo program was established further to calculate the detailed recoil range distribution and the recoil probability (emanating power). The powerful Turning Bands Method (TBM) of random field is applied to simulate the 3-D porous texture based on the porosity and the correlation function of the porous texture. Based on the simulated porous texture, the fractal dimension of the surface is calculated and used to calculate the effective surface area for radon recoil. The relations between the air buffer thickness, embedding effect of recoil, and the measuring scale of the surface area for the porous texture are discussed and numerically calculated. After these calculations are performed, the relations between the emanating rate, surface area, material density, and porosity are established to calculate the radon emanation rate from porous materials. This paper provides a clear theoretical picture of the mechanism of radon release from the building materials. It has also potential application to the recoil release calculations of other radioactive elements from solid materials.
预测建筑材料中的氡释放是一个普遍问题。由于通过实验方法追踪每条反冲氡路径并测量多孔结构的表面积是不切实际的,因此本文采用了一种强大的计算机模拟方法。基于物质中离子传输的动量和能量守恒的蒙特卡罗模拟程序TRIM被修改,以在三维框架中模拟反冲路径。进一步建立了一个后续蒙特卡罗程序,以计算详细的反冲范围分布和反冲概率(析出率)。基于多孔结构的孔隙率和相关函数,应用强大的随机场转动带方法(TBM)来模拟三维多孔结构。基于模拟的多孔结构,计算表面的分形维数,并用于计算氡反冲的有效表面积。讨论并数值计算了空气缓冲层厚度、反冲嵌入效应与多孔结构表面积测量尺度之间的关系。进行这些计算后,建立析出率、表面积、材料密度和孔隙率之间的关系,以计算多孔材料的氡析出率。本文提供了建筑材料中氡释放机制的清晰理论图景。它也可能应用于固体材料中其他放射性元素的反冲释放计算。