Mederski W W, Dorsch D, Bokel H H, Beier N, Lues I, Schelling P
Department of Chemistry, E. Merck, Darmstadt, Germany.
J Med Chem. 1994 May 27;37(11):1632-45. doi: 10.1021/jm00037a014.
A series of novel non-peptide angiotensin II receptor antagonists containing a 2,3,5-trisubstituted 4,5-dihydro-4-oxo-3H-imidazo[4,5-c]pyridine was prepared via several synthetic routes. Their affinity for angiotensin II receptors was established in a binding assay experiment and in an isolated-organ test. Molecules with small alkyl groups at C-2 and the (methylbiphenylyl)tetrazole moiety at N-3 were the preferred compounds with affinities and potencies in the nanomolar range. Variations at the N-5 position modulate the activity. Substitution at N-5 with various benzyl groups led to derivatives with in vitro potencies in the nanomolar range, which were equivalent to those of losartan in these assays. Replacement of the N-5 hydrogen with acetic acid esters or, in particular, acetamides gave molecules with increased activity. The most potent was 2-butyl-4,5-dihydro-4-oxo-3-[[2'-(1H-tetrazol-5-yl)-4- biphenylyl]methyl]-3H-imidazo[4,5-c]pyridine-5- (N,N-diethylacetamide) (14u), which is superior to L-158,809 in vitro. Two prototypes were selected as their potassium salts for in vivo testing as antihypertensives. Compounds 14a (EMD 61,650) and 14q (EMD 66,684) reduced blood pressure dose dependently in spontaneously hypertensive rats when administered iv. In this assay, acetamide 14q is superior to losartan.
通过几种合成路线制备了一系列含有2,3,5-三取代的4,5-二氢-4-氧代-3H-咪唑并[4,5-c]吡啶的新型非肽类血管紧张素II受体拮抗剂。在结合试验和离体器官试验中确定了它们对血管紧张素II受体的亲和力。在C-2位带有小烷基且在N-3位带有(甲基联苯基)四唑部分的分子是优选的化合物,其亲和力和效能在纳摩尔范围内。N-5位的变化调节活性。用各种苄基在N-5位进行取代得到了在这些试验中体外效能在纳摩尔范围内的衍生物,其与氯沙坦相当。用乙酸酯特别是乙酰胺取代N-5位的氢得到了活性增加的分子。最有效的是2-丁基-4,5-二氢-4-氧代-3-[[2'-(1H-四唑-5-基)-4-联苯基]甲基]-3H-咪唑并[4,5-c]吡啶-5-(N,N-二乙基乙酰胺)(14u),其在体外优于L-158,809。选择了两种原型作为其钾盐进行体内抗高血压测试。化合物14a(EMD 61,650)和14q(EMD 66,684)静脉注射给药时能使自发性高血压大鼠的血压剂量依赖性降低。在该试验中,乙酰胺14q优于氯沙坦。