Wallace L
National Exposure Research Laboratory, U.S. Environmental Protection Agency, Warrenton, Virginia.
J Air Waste Manag Assoc. 1996 Feb;46(2):98-126. doi: 10.1080/10473289.1996.10467451.
This paper reviews studies of particle concentrations and sources in homes and buildings. Three major studies of indoor and outdoor concentrations in U.S. homes are summarized in detail and compared. A number of smaller studies in homes are also briefly summarized. One study of 38 buildings and several smaller studies of buildings are also reviewed. All major studies found that an important indoor source of fine and coarse particles was cigarette smoking, with estimated increases in homes with smokers ranging from 25 to 45 micrograms/m3 PM2.5. Several studies identified cooking as a second important source. All of the three major studies found a substantial portion of indoor particles to be due to unexplained indoor sources, suggesting a topic for future research. One study also found a large unexplained increase in personal exposure to PM10 compared to concurrent indoor or outdoor concentrations--the so-called "personal cloud," a second topic for further research. The impact of outdoor air particles on indoor concentrations was considered. Equilibrium mass balance models indicate that this is a function of the penetration P through the building envelope, the air exchange rate a, and the particle decay rate k. EPA's PTEAM Study provided an estimate for k of 0.39 h-1 for fine particles and 1.01 h-1 for coarse particles. Two studies suggest that P = 1 for PM10. Using these results, the fraction of outdoor air PM2.5 and PM10 particles found indoors at a given air exchange rate can be calculated. The protective effect of reducing air exchange rates during periods of high outdoor particle pollution can thus be quantified.
本文综述了有关家庭和建筑物内颗粒物浓度及来源的研究。详细总结并比较了美国对家庭室内外浓度进行的三项主要研究。还简要总结了一些针对家庭的小型研究。同时也回顾了一项对38座建筑物的研究以及几项针对建筑物的小型研究。所有主要研究均发现,室内细颗粒物和粗颗粒物的一个重要来源是吸烟,据估计,有吸烟者的家庭中PM2.5浓度增加范围为25至45微克/立方米。多项研究将烹饪确定为第二个重要来源。三项主要研究均发现,很大一部分室内颗粒物来自不明室内来源,这为未来研究提出了一个课题。一项研究还发现,与同时期的室内或室外浓度相比,个人接触PM10的量出现了大幅不明增加——即所谓的“个人云”,这是另一个有待进一步研究的课题。文中考虑了室外空气颗粒物对室内浓度的影响。平衡质量平衡模型表明,这是穿透建筑物围护结构的渗透率P、空气交换率a和颗粒物衰减率k的函数。美国环境保护局的PTEAM研究给出的细颗粒物k值估计为0.39小时-1,粗颗粒物为1.01小时-1。两项研究表明,PM10的P = 1。利用这些结果,可以计算出在给定空气交换率下室内发现的室外空气PM2.5和PM10颗粒物的比例。因此,可以量化在室外颗粒物污染严重期间降低空气交换率的保护作用。